THE DETERMINATION OF THE CRYSTAL STRUCTURE OF ACETYLTRIPHENYLGERMANE BY X-RAY DIFFRACTION by ROY WILLIAM HARRISON B.Sc., University of B r i t i s h Columbia, 1965 A THESIS SUBMITTED IN PARTIAL FULFILMENT OF THE REQUIREMENTS FOR THE DEGREE OF MASTER OF SCIENCE i n the Department of Chemistry We accept t h i s thesis as conforming to the required standard. THE UNIVERSITY OF BRITISH COLUMBIA . July, 1967 In p r e s e n t i n g t h i s t h e s i s i n p a r t i a l f u l f i l m e n t o f the r e q u i r e m e n t s f o r an advanced deg ree a t the U n i v e r s i t y o f B r i t i s h C o l u m b i a , I ag r ee t h a t the L i b r a r y s h a l l make i t f r e e l y a v a i l a b l e f o r r e f e r e n c e and s t u d y . I f u r t h e r ag r ee t h a t p e r m i s s i o n f o r e x t e n s i v e c o p y i n g o f t h i s t h e s i s f o r s c h o l a r l y p u r p o s e s may be g r a n t e d by the Head o f my Depa r tmen t o r by h i s r e p r e s e n t a t i v e s . I t i s u n d e r s t o o d t h a t c o p y i n g o r p u b l i c a t i o n o f t h i s t h e s i s f o r f i n a n c i a l g a i n s h a l l no t be a l l o w e d w i t h o u t my w r i t t e n p e r m i s s i o n , Depa r tment The U n i v e r s i t y o f B r i t i s h C o l u m b i a V a n c o u v e r 8, Canada - 11 -ABSTRACT ' Acetyltriphenylgermane, (C^H^J^GeCOCH^, c r y s t a l l i z e s i n the monoclinic system with a = 15.30s b = 14»53j» c. = 7.6S A, and ^» 94.3 . The space group i s and there are four molecules per unit c e l l , thus each molecule forms an asymmetric unit i n the c e l l . The i n t e n s i t i e s of 2537 r e f l e c t i o n s were measured by means of a s c i n t i l l a t i o n counter using CuKcc ra d i a t i o n . The structure was determined by heavy atom Patterson and Fourier synthesis and refinement was by least-squares methods. The f i n a l discrepancy, R, f o r 1334 observed r e f l e c t i o n s i s 0.075. The compound was found to be tetrahedral about the germanium atom, with only small deviations caused by the spreading of the phenyl rings. The phenyl rings are planar with a mean C-C bond distance of 1.3#3 A, mean C-C-C bond angle of 120.0°, and a mean C-H bond distance of 1.09^ A. Interraolecular i n t e r a c t i o n causes one ring to deviate from a symmetric propeller orientation. Two Ge-C bond distances were found: Ge~Cphenyl distance o o of 1.945 A and G e - C a c e t y l distance of 2.011 A. The longer Ge-C bond i s attributed to contribution from a resonance structure i n which there i s no formal bond between germanium and the carbonyl carbon, r e s u l t i n g i n a p a r t i a l negative charge.on the oxygen and a p a r t i a l p o s i t i v e charge on the germanium. This i s supported by the electronegativity difference between carbon and germanium. The C=0 bond distance i s 1.20 AQ - i i i -TABLE OF CONTENTS PAGE T I T L E PAGE . . . . . . . . . . . . . . . . . . i ABSTiriACT o o o * * o « « * o * o « o o • * • « « « • « "XI. TABLE OF CONTENTS . . . . . . . i i i L I S T OF TABLES i v L I S T OF F IGURES . . i . . v ACKNOWLEDGEMENTS . . . • • • • v i INTRODUCTION . . . . . . . . . . . . . . 1 EXPERIMENTAL 4 STRUCTURE ANALYS I S 5 COORDINATES AND MOLECULAR DIMENSIONS . 9 DISCUSSION 16 BIBLIOGRAPHY 1 20 APPENDIX I. TABLE OF OBSERVED AND CALCULATED STRUCTURE FACTORS . . . . . . . 21 _ i v -LIST OF TABLES TABLE PAGE I- F i n a l p o s i t i o n a l parameters and standard deviations . . . . . . 10 II * F i n a l thermal parameters and standard deviatxons . . . . . . . . . . . . . . . . . 11 I I I . Equations of mean planes and angles between IV. Bond distances and angles with standard deviations . . . . . . . . . . 13 V 0 Shorter intermolecular distances . . . . . . 14 VI. Comparison of carbonyl stretching frequencies and electronegativity of o c-substituent . . . IS VII. Observed and calculated structure factors . 2J. - v -LIST OF FIGURES FIGURE PAGE 1. Perturbation of the energy l e v e l s of carbonyl by s i l i c o n . . . . . . . . . . . . 2 2. (a) Projected electron-density d i s t r i b u t i o n . . S (b) Perspective drawing showing atom numbering , $ 3. Molecular packing diagram 15 ~ v i -ACKNOWLEDGMENTS. I would l i k e to express my appreciation f o r the guidance and encouragement given to me by Dr. J, Trotter during the progress of t h i s work. I am also indebted to Dr. K. Yates f o r the c r y s t a l samples of the <*.-silyl and oc-germyl ketones-which he has provided* / / - 1 -INTRODUCTION . I n v e s t i g a t i o n s of the s p e c t r a l a c t i v i t y of the s i l y l and oC-germyl ketones (1-4) have shovm these compounds to d i f f e r markedly from t h e i r carbon analogues. The u l t r a v i o l e t spectra of b e n z o y l s i l a n e s are c h a r a c t e r i z e d by absorption at about 403-417 iy-, a s c r i b e d to a n-fi t r a n s i t i o n of the carbonyl group, i n v o l v i n g i n t e r a c t i o n w i t h the 3 d - o r b i t a l s of the s i l i c o n atom. A c e t y l s i l a n e s have absorption about 360-370 m^ w h i l e carbon analogues absorb at $0-100 m/i- shorter wavelength than the corresponding s i l i c o n compound. At the same time, the i n f r a r e d carbonyl s t r e t c h i n g v i b r a t i o n i s at a very low frequency: 1613 cm"-'- (6.1S/4 f o r benzoyl- and 1645 cm~l (6.OS//) f o r a c e t y l s i l a n e s , w h i l e the carbon analogues absorb at about 1636 cm"! (5.93/^) and 1715 cm-1 (5.33/4 r e s p e c t i v e l y . For o<.-germyl ketones, the s h i f t i n frequency i s o n l y s l i g h t l y lower. The positions of these absorption bands are r e l a t i v e l y i n s e n s i t i v e to the groups attached to s i l i c o n o r germanium. The f i r s t attempt to e x p l a i n the abnormal s p e c t r a l character of the o L - s i l y l and ©c-germyl ketones was made by Brook et a l (2) who a t t r i b u t e d the l a r g e i n f r a r e d s h i f t i n -c x - s i l y l ketones to the i n t e r a c t i o n between lone p a i r e l e c t r o n s on the carbonyl oxygen and vacant 3 d - o r b i t a l s on the s i l i c o n (^-tr bonding). This diT-ptr bonding would d i s t o r t and s t r e t c h the carbonyl group by t r a n s f e r of e l e c t r o n d e n s i t y toxrards the s i l i c o n atom, r e s u l t i n g i n a lowered fo r c e constant and thus a s h i f t i n the carbonyl s t r e t c h i n g v i b r a t i o n t o longer - 2 -wavelengths. West and Harnish (5) s i m i l a r l y interpreted the u l t r a -v i o l e t absortion spectra, using d-orbitals on the s i l i c o n , but i n terms of resonance interaction between the si l i c o n , atom and the lY-orbitals of the carbonyl group,pas shown i n f ' i g . l . 0 = C 0=C-SL TT /l V 7 -ML F i g . 1. Perturbation of the energy l e v e l s of. carbonyl by s i l i c o n , t r a n s i t i o n (n-ff ) results from t r a n s i t i o n s^if-p^ — S Q T P P 0 T T * where Tr*" i s the antibonding 1Y l e v e l . More recently, Brook, Kiv i s i k k , and LeGrow ( 6 ) , studying the spectral properties of p-substituted benzoyl-triphenylsilanes, concluded that the low infrared carbonyl stretching freo.uency i n benzoylsilanes was a result- of si g n i f i c a n t single-bond character i n the carbonyl group caused by the inductive release of electrons by. the adjacent s i l i c o n atom. In support of t h i s , Yates and Agollni (4) showed, the order of base strength to be I^SiCOPh£ R^GeCOFh > R^CCOPh, and Brook and Pierce.(7) shov:ed. that but not K'-silyl ketones absorb at lower frequency than t h e i r carbon - 3 -analogues. Thus, i n the ground state, o c - s i l y l and .<*-germyl ketones must have a s i g n i f i c a n t negative charge associated with the carbonyl oxygen atom, which i s consistent with contribution from a structure of the type + / 0 R 3 X - C ^ X P h To our knowledge, no crystallographic studies had been done on compounds of t h i s type, and a l i t e r a t u r e survey produced no X-C or C=0 bond lengths f o r them. It was f e l t that, i n 'such an investigation, i f accurate, bond lengths could be obtained, evidence for or against p a r t i c i p a t i o n of the d-orbitals of the s i l i c o n or germanium i n the bonding would be found i n a study of the bond lengths. The compound chosen was.acetyltriphenylgermane, which has a carbonyl stretching frequency at 1669 cm"-'- and peaks at 352, 365, and 3^0 m/t i n the u l t r a v i o l e t spectrum (3). 0 -. 4 -,EXPERIMENTAL . ' • C r y s t a l s of a'cetyltriphenylgermane are white needles elongated along c.. The den s i t y was measured by f l o a t a t i o n i n aqueous potassium'iodide and th e u n i t c e l l dimensions and space group were determined from r o t a t i o n , Weissenberg, and precession f i l m s , and. on the G. E. Spectrogoniometer. C r y s t a l Data (-AjCuK*. = 1.5413 A; X,M0K*. = 0.7107 A) Acetyltriphenylgermane, (C5H5 J^GeCOCH-j; mol. wt-. 346.9, ra. pt. 121.5 - 123.0°. M o n o c l i n i c , a = 15.30±0.02, b - 14.53^0.02, c - 7.68± 0.02, f = 9 4 . S ± 0.3°. Volume of u n i t c e l l = 1704 P . D x (Z = 4) = I.35 g. cm.-3. . D m = 1.36 g. cm.~3. Absorption c o e f f i c i e n t f o r CuK^ X-rays, A= 1.541$ A, /"-s 26.4 cm.-1.• Absorption c o e f f i c i e n t f o r MoK^X-rays, ?V- 0.7107 A, y U = 19.0 cm."1, .Absent r e f l e c t i o n s : h0^ when-t i s odd OkO when k i s odd. Space group: P2^/c ( C ^ ) . T o t a l number of e l e c t r o n s per u n i t c e l l : F(000) = 712. The i n t e n s i t i e s of the r e f l e c t i o n s were measured on a General E l e c t r i c Spectrogoniometer, w i t h Single C r y s t a l Q r i e n t e r , s c i n t i l l a t i o n counter, approximately monochromatic CuK^ r a d i a t i o n being obtained by use of a n i c k e l f i l t e r and pulse height analyzer. A l l 2537 r e f l e c t i o n s i n the range 0< 29-^120° (corresponding to a minimum interplanar 0 spacing d =. 0 ,89.A) were examined, and 1^34 (72%) had an i n t e n s i t y above background. The 703 unobserved r e f l e c t i o n s were included i n the l a t t e r stages of the structure analysis with • |FQI = V 0 . 4 Zthreshold* i n t e n s i t i e s were corrected for background (approximately a function of 9 only). The c r y s t a l used f o r recording the i n t e n s i t i e s had dimensions 0.2 x 0.25 x 0 . 4 mm and-was mounted with c* p a r a l l e l to the. axis of the goniostat. No absorption corrections were applied. Lorentz and pol a r i z a t i o n corrections were applied and structure amplitudes derived. -STRUCTURE ANALYSIS The position of the germanium atom was determined from a three-dimensional Patterson synthesis as (0.7375, 0.5271, 0 . 3 1 4 6 ) . Structure factors were calculated f o r a l l the r e f l e c t i o n s using the scattering factors f o r Ge (corrected f o r anomalous dispersion) from the International Tables (9) and a temperature factor, B, of 3-0 A^ ?(R = 0 . 3 4 ) . A three-dimensional Fourier series was summed with the signs of the structure amplitudes based on the germanium atom contribution. Peaks corresponding to a l l of the atoms (except hydrogens) appeared on the electron density map. The oxygen atom was distinguishable from the methyl carbon by both peak height and. bond distance. The structure "factors for a l l 22 atoms were calculated (R = 0 . 2 4 ) , setting - 6 -B = 3,0 for a l l atoms and using the C and 0 scattering factors from the International Tables ( 9 ) , The positional and i s o t r o p i c thermal parameters and an o v e r a l l scale f a c t o r were refined by block diagonal least-squares methods. The function minimized was £,w(F 0_F c) 2, withVw~=.0 f o r unobserved r e f l e c t i o n s , Vw - 1 when I F Q I ^ 1 5 , and Vw" = 15/ Zo when |Fj0|>15o Several cycles of least-squares refinement reduced R to 0.0#7. A comparison of the calculated and observed structure factors showed twenty-five r e f l e c t i o n s , including the following strong " '•. refle c t i o n s ' (311, 402, 212), had serious disagreement',. Of these, eleven were corrected by comparison with films and the rest, a l l very weak r e f l e c t i o n s , were removed from the least-squares refinement. Following several more l e a s t -squares cycles, a ( F Q - Z C ^ difference synthesis was computed to locate the hydrogen atoms. A l l f i f t e e n phenyl hydrogens were located, but one of these, H{26), gave a C-H bond o distance of 0.67 A and so was placed at i t s t h e o r e t i c a l position. Attempts to locate the methyl hydrogens were unsuccessful. Further refinement, including the hydrogen-, atoms at fixed positions and with B = 6*5 A , reduced R to 0.073. At t h i s stage, an analysis of the values of (Fo-F c) suggested a more appropriate weighting scheme: V"w" - ; 1 , The unobserved r e f l e c t i o n s were also included,v.with - 7 - ' IFQI = V0.4 ^threshold and were given a weight V™-*3 0.62. The average w(F 0-F c) was novr approximately constant over a l l values of F Q taken at i n t e r v a l s of 5. Refining all°-37. atoms with the new weighting scheme changed R to 0.077. Ge, 0, C (3 ) , 0(4), C(5), C ( l l ) , and C(l7) were then refined f o r three cycles with anisotropic temperature factors, the hydrogens being fixed i n t h e i r best position (peak position or f i r s t or second refinement position) according to bond length a f t e r the f i r s t cycle, and the remaining carbon atoms being fi x e d i n position after the second cycle, reducing R to 0.073. A f i n a l structure factor calculation, including the 14 r e f l e c t i o n s that were removed from the refinement, gave R - 0.075. The f i n a l measured and calculated structure factors are l i s t e d i n Table VI.(Appendix I ) . A f i n a l three-dimensional Fourier series was summed and superimposed sections of the re s u l t i n g electron-density d i s t r i b u t i o n are shown i n Figure 2, together with a drawing of the structure giving the atom numbering used i n the analysis. A f i n a l o difference map showed maximum fluctuations bf ± 0.5eA">. (a-) Electron-density projection along the c axis. Contours are at intervals of 1 e. sta r t i n g at 2' e. A"*^ for carbon, and of 10 e. A-3 s t a r t i n g a t f o r Ge. 10 e. (b) Perspective drawing o f the structure giving, the numbering used, - 9 -COORDINATES AND MOLECULAR DIMENSIONS The f i n a l p o s i t i o n a l p a r a m e t e r s and t h e i r s t a n d a r d d e v i a t i o n s a r e g i v e n i n T a b l e I. x , Z> a n d z. a r e f r a c t i o n a l c o o r d i n a t e s r e f e r r e d t o t h e m o n o c l i n i c c r y s t a l a x e s ; c r ( x ) , c r ( y ) , a n d c r ( z ) a r e t h e s t a n d a r d d e v i a t i o n s o f t h e o c o o r d i n a t e s ( i n A) c o m p u t e d f r o m t h e l e a s t - s q u a r e s r e s i d u a l s . The p o s i t i o n s o f t h e h y d r o g e n a toms a r e l e a s t a c c u r a t e l y d e t e r m i n e d and a r e n o t c o n s i d e r e d f u r t h e r . T a b l e I I g i v e s t h e f i n a l t h e r m a l p a r a m e t e r s , where Uj.j a r e t h e c o m p o n e n t s o f t h e v i b r a t i o n t e n s o r s , w r i t t e n i n m a t r i x f o r m , and r e f e r r e d t o t h e a x e s a * , b * , and c * . The e q u a t i o n s o f t h e mean p l a n e s o f t h e t h r e e p h e n y l r i n g s a r e g i v e n i n T a b l e I I I , a l o n g w i t h t h e p l a n e s t h r o u g h C(3 ) - G e - C ( p h e n y l ) and t h e i n t e r p l a n a r a n g l e s . Bond d i s t a n c e s and v a l e n c y a n g l e s t o g e t h e r w i t h t h e i r s t a n d a r d d e v i a t i o n s a r e l i s t e d i n T a b l e - I V , and T a b l e V l i s t s a l l t h e c r y s t a l l o g r a p h i c a l l y o i n d e p e n d e n t i n t e r m o l e c u l a r d i s t a n c e s s h o r t e r t h a n 3.8 A . Two i m p o r t a n t d i s t a n c e s i n v o l v i n g t h e C ( l l ) - C ( l 6 ) r i n g s a r e a l s o l i s t e d . F i g u r e 3 i l l u s t r a t e s . t h e p a c k i n g o f t h e m o l e c u l e s . - 10 -Table I Final positional parameters (fractional) And standard deviations (A). Atom X Z z Ge>Si. The electro-n e g a t i v i t i e s determined by A l l r e d and Rochow ( l l ) support t h i s as shown i n Table VI, i n which the trend i n the carbonyl Table VI „ Comparison of the carbonyl stretching c frequencies and the electronegativity of the oc-substituent. ; Compound C=0 stretching f r e q . (cm~l) Electronegativity 2.50 2.02 1.74 stretching frequency i s closely p a r a l l e l e d by that of the el e c t r o n e g a t i v i t i e s . While these el e c t r o n e g a t i v i t i e s are s t r i c t l y only those of the i s o l a t e d atom, since the environment of the oC-substituent i s i d e n t i c a l i n each compound t h e i r ^ 3CCOCH 3 1721 (2) ^3GeCOCH3 1669 (3) ^ 3Sicoce 3 1645 (2) - 19 -r e l a t i v e values should be correct.. These trends suggest that the S i - C a c e t y - ^ bond i n the analogous s i l i c o n compound should be r e l a t i v e l y longer than the corresponding bond i n the germanium compound and a structure analysis of acetyltriphenylsilane would be useful i n supporting the bonding scheme which has been proposed f o r the o<-germanium ketone* / - 20 -BIBLIOGRAPHY 1 0 A. G0 Brook, Am. Chem, Soc. 22,'. 4373 ( 1 9 5 7 ) . 2. A. G. Brook', M. A. Quigley, G0 J. D. Peddle, N. V a Schwartz., and C 0 M. Warner, J. Am. Chem. Soc. 82, 51.02 ( I 9 6 0 ) . • 3„ A. G. Brook and G. J„ D, Peddle, J. Organometalo!'.Chem0 2, 106 (1966). • 4 . K. Yates and F 0 A g o l i n i , Can. J. Chem. L 4 5 2229 (1966) 5o D. F. Harnish and R. West, Inorg. Chem. 2, 1082 (1963) ' 6 a A. G0 Brook, R. Kivi s i k k , and G. E„ LeGrow, Can. J. Chem. i i , 1175 (1965). 7. A. G. Brook and J. B 0 Pierce, Can. J . ' Chem. 4 2 , 293 (l964)o 3. G. J. Peddle, J. Organometal. Chem. 436 (1966). 9. International Tables f o r X-ray Crystallography, Vol. I l l Kynoch Press (1962). 10c V . W. Laurie, J . . Chem. Phys. 3 0 , . 1210 ( l 9 5 9 ) o 11. F. A. Cotton and G. Wilkinson, "Advanced Inorganic Chemistry", Wiley, New York (1962). - 21 -APPENDIX I Table VII" Observed and Calculated Structure Factors {* indicates a r e f l e c t i o n which was not included i n the least-squares refinement. Negative F Q values indicate an unobserved re f l e c t i o n . ) - 22 -Table VII 0 1 1 6 8 . 3 73.7 -14 7 11.4 -8.7 2 73.1 69.8 -J 15" 2 15.2 - 1 8 . 2 hk -I ! V 152.ft 1 71.9 -144.4 75.4 15 7 -15 7 -2.2 -2.7 4.7 0 . 3 'I \ 36. ft 31.C 36. 1 29.7 -4 IC 7 19. C 2 9.5 17.5 -12. t 1 Fo Z 1 1 2 7 . * 27.7 0 9 7.7 -6.2 - 3 2 25.8 -12.7 5 tC 2 -2 .7 -0.6 1 " l 1 1 AC.2 1 132.8 -AC.7 144.5 I 9 -I 9 7.1 26. 7 7.1 25.8 j 1 1 1 . ! 72.7 - l U . a - 7 1 . 3 -5 tC 6 IC 2 18.6 2 19.C 19.4 -2C.5 t c 0 2.1 1 A3.3 -59.7 2 9 - 1 . 9 C O 4 i . e -31. t -6 IC 2 14.4 13.7 X c 9 c c 0 143.4 5.5 -148.1 -10 .2 -1 ! I 7ft.8 1 T9 .4 70 . 3 75.9 -2 9 3 9 -1 .5 13.9 -2.7 -13.3 \ 73.4 44.8 7 3 . 3 BC.6 7 tC - 7 IC 2 -2.2 2 -2.2 1.7 9.2 4 0 c 7 .9 - A . 4 + 9 1 1 ae. e - 8 5 . T -3" 4 -4.1 -6 2 27.1 27. t B IC 2 - 7 . 2 1 .5 * c « c c c 22.e 26.7 -19.9 -24.5 ~l ! 1 38 .7 1 9.4 38.6 C.C • 4 « -4 9 -1.9 n.s 1.7 13.A -1.7 I 79.5 3.C -60.8 -8 IC 9 IC 2 7.5 7 - 2 . 7 -5.6 -3.2 1 t c 9.ft -T.4 1 40.3 -48. ft 9 9 -2 .C - 2 . 9 47.5 -44.8 -9 IC ? 14.2 - 1 5 . 3 a c « c a 0 24. 8 2C.5 24.A -19.4 -T 1 1 81.1 I 3ft.ft 11.7 -37.6 -5 9 6 9 -2 C -2.1 l .C - C Z I - 1 . 9 I - 1 . 5 -C .6 1 . 3 10 IC -10 IC 2 -2.5 2 1 C 5 3.C *.9 10 c c 45.C -45.4 9 1 1 16.3 -33 .1 -6 4 14.1 -lfc.2 -9 2 2 3 C 8 5 1 . 2 11 IC 2 -2 .4 -7.2 11 c 0 4 * .9 49 .A —8 1 1 24. C 24.C 7 9 -7.1 2.8 10 2 ! 17.« 34.2 -11 IC 2 11.4 1ft. 1 12 C a i f .e 21.3 . < 1 1 49.3 -45.2 - 7 9 -2.1 -4.2 - 10 2 I 2C.ft -20.0 12 tC 2 - 7 . 2 -1.5 13 t d 43.C -4C.4 1 17.9 11.C a 9 -2.2 1-3 2 ft.8 3.3 -12 IC 2 -2.1 -7.0 1* c IS C c c 9.2 2ft.1 -4 .7 24. 1 -10 1 1 19.2 1 48.2 U . 5 -46 . 1 ~ H 9 9 9 - 2 . 2 7.8 -2.2 -6 .0 " l 2 ] t 42.1 2 32.4 -42.9 -10.C -13 IC 0 17 2 -1.2 2 2*. 1 -4 .0 21. C 16 C IT C c 5^1 22.C - a . 5 -20.4 -11 1 1 92.5 I 9.9 46.5 -8.3 -•) 9 10 9 -2.2 11.1 1.9 10.8 "15 5 2 75.3 2 8.7 25.2 8.9 1 17 -1 12 2 IC.ft 2 - 2 . 2 8.7 -5.1 0 2 c 119.C 115.A 1? 1 1 23.3 -22.a -10 9 5.4 89 - 1 3 2 2 2 9 . 1 10.1 2 17 2 71.4 -70.5 t 2 4.2 2.C 1 92. C 51.2 U 5* - 2 . 2 .7 2 23.7 74.5 -2 17 2 8 . 4 -11.3 2 2 3 2 5 121.9 JC.4 -118.9 10.4 - 1 J 1 1 2C.7 I -2 .5 -JI.3 -4 .7 -11 « 12 9 7.9 -2.4 - 2 . 8 -2 .4 "!? I 7 8.9 2 11.5 -8.4 -t l.7 3 17 -3 12 2 11.7 2 -2.2 -9.4 6 . 3 4 Z 9 2 69 . 7 49.C 72.C . -46.5 - i l l 1 25.3 1 44.4 25.a -42.1 -12 4 13 9 -2.5 -2.3 -0.7 -3 .9 2 .14.5 2 14.5 -17.7 -15.7 4 12 -4 12 2 5.1 7 - 2 . 2 9.0 . - 7 . 2 A 2 c 79.2 -74.7 i s l I - 2 .5 5.6 -13 9 - 2 . 4 - 1 . 4 - 16 2 2 -2.3 6.4 5 12 2 - 2 . 2 3.7 7 2 4 9 . 9 « . « I I I . C 10.9 14 4 -2.1 -3.8 2 44.9 -49.5 - 5 . 1 2 2 5.9 -8 . I' 1 2 « 2 I 44. ft SC.9 43.4 -J3.1 -it ! 1 M . J 1 21.A -19 ,4 22.1 -14 9 0 11 -2.2 - 2 . 1 - 4 . 4 -0.2 .{ ; ? 75.9 i 74.8 -75.5 8C.9 6 12 -6 12 -2.22 12. ft -t5.5 13.5 1C 2 11 2 13.5 H . C -14.1 31.4 1 I - 2 . 2 1 9.5 -».i 2.a 1 11 -1 11 19.7 8.1 20.3 -6.1 .5 J 2 57.5 ? t.e 54.6 - 3.4 7 12 -7 12 2 -2.2 2 It.5 - 2 . 3 9.7 12 2 c 22. ! 18.1 t 3 1 1 U . 4 -113.3 2 11 -2.1 1.3 3 2 61.4 55.4 8 17 2 9.1 7.5 IS 2 1ft.4 -11.4 I 98.7 99.6 - 7 11 -2.1 -0 .8 2 59.1 -56.3 -8 12 -2 5 -2.9 14 2 c IC.4 -10.5 2 3 [ 96.A -93.7 3 It 21.4 -7^.5 4 2 83 .4 -77,5 9 12 2 -2.1 1 619 2 c 25.9 2 5 . 3 —2 1 1 19.3 -40.2 -3 11 7.5 7.4 . 4 2 71.9 -2 J.C -9 12 2 1C.7 -12.1 It 2 17 a I -2 .3 21.7 1.9 -2C. ) _\ \ 1 *0 .2 i e.9 82.9 - 3 . C 4 11 -4 11 -7.2 7.5 -3.7 -8.1 . * 7 J l . 12 6 7 . 3 -28.8 44.7 .10 12 - 10 12 2 5.7 2 -2.3 "8.6 3 . 3 0 * 47.2 -42.1 4 ) 1 A.C -6.9 9 11 5.8 8.5 6 2 3 C C 31.1 -11 12 2 12. t 11.1 2 * 2 4 . ; i t . 2 25.9 -B4.4 9 1 I 7.5 1 94 .7 4.8 -89.2 -3 11 6 11 ice 12.1 -11.5 -11.6 _ 7 2 42. C 2 -1 .8 4 4 . C 4.1 0 14 2 14.1 7 2C.2 14.1 I H . C I 4 c -1.2 C.4 - 9 J i «2 .e 64.3 -6 It -2.2 -C.5 -7 2 2 C 7 -29.8 -t (4 2 14.C -12.8 4 4 9 4 I 99.C 42.8 62.4 -41.C -6 1 1 13.3 1 93.a 14.1 -5).7 7 11 - 7 11 - 2 . 2 1.C - -1.6 -ft.4 8 -8 2 ice 2 8.2 -29.7 -8.C -7 l l* 2 11.4 2 i.e -11.7 -7.8 6 4 47.C -44.2 1 51 .7 54.4 B 11 • 7.9 -/.a 9 2 -Z.C 0.8 2 17.1 -15.9 7 * 8 4 $ AC.2 39. 1 59.4 4C.9 "a i I 2ft.7 1 26.2 -30.0 -28.4 -8 I 1 9 t l 11.ft - 2 . 2 -11.4 7.5 -9 to ; 2 4 3 . 4 7 12.5 43.3 I t . 2 "4 " 7 17. f 2 16.8 65 15.7 9 4 c 35. 9 -44.8 - a ' i 1 67.5 69. 2__ -9 U 7.5 10. c -10 2 9.2 -7.4 -4 M 2 -2.4 4 . 3 10 4 11 4 1 7 2 7 . 3 -31.1 27.C -9 3 I 35.3 1 17.7 - 3 8 . 3 17.7 10 1 1 -10 11 -2.4 1 17.5 7.C 16.7 11 -11 ft.92 3 3 . 4 - IC. 7 -34 .c -I !« 2 -2.1 7 14.8 C.2 -lt.fi ** * 22. e 22.2 1 29 .4 29.9 11 11 -2.3 -0.7 12 2 14.ft -21.4 2 1C.7 -9.4 "n * 14 4 I 19.1 -2.2 -11.9 -1.6 T i 3 1 44 . 3 1 31.4 -45.2 3 0 . 9 -11 11 12 1 1 7.3 1 -2.2 7.4 1.1 -17 13 * 2 14.1 2 17.7 13.2 12 . 1 "* !J 2 8 . 2 2 -2.2 -ft.e -C.6 19 4 19.2 19.1 -11 3 1 - 2 . 3 -2.2 -12 11 I -2.2 0.2 -13 2 n . e IB.8 -T 1 * 2 1 2 . e 13 . 1 1ft 4 0 ft -2.? 7*.9 2.9 71.5 -12 1 1 9.2 1 41.1 - 7 . 1 37.4 a i i 1 13 1 -2.2 2C.7 1.7 20.6 14 -14 j 2 2 3 . 2 2 -2.5 2 2 . 2 -4.1 ' l 2 -2.1 3 79.4 - C t -80.7 I t 4.5 4.4 1 17.7 -19.e -I 13 I 21.2 -21.6 15 2 - 2 . 3 - 7 . 3 1 49.1 41.3 2 ft 3 e. I 39.1 14.9 -38. ft -12 .7 ' l l 1 I 14 . 2 1 14.1 -12.7 1C.7 2 1! -2 13 t tt.e 1 18.7 -B.6 17.7 -15 -16 I 2 12. C 2 t l.7 -10.9 I C C 2 1 3 4.7 1 51.5 7 1 52. S 4 A 44 .9 42.1 • - 1 * J 1 21.7 -20.6 3 13 1 24.5 -22.9 0 t 2 5 7 . 4 -54 .4 -2 1 1 48.5 fr9.ft 9 £ 6 ft 12.1 22.9 - t l . 9 -21 . * > 1 i t . ; t -2.3 t4.2 2.6 -3 13 4 1! 1 It.2 1 - 2 . 2 14.A3.2 1 I 2 I C C 2 7.4 -14.C 7.9 - 1 1 1 JC.1 1 5.5 -54.4 -1.8 T e 1 r.c 14.9 1 14.ft -15.3 -4 13 1 15.ft -15.1 2 2 41.5 4 1 . 3 3 14.8 -17.5 a « 9 « I 32.9 22. C 32.4 -19.e 1 22.ft 1 25 .7 20.4 -25.7 9 1 1 -5 13 1 I C S 1 -2.2 11.B -1 .8 -2 3 2 19.C 2 14.4 19.6 14.7 "5 1 1 81.4 3 29 . E -01.C 5Cf i 10 * c 3 7 . 9 -39 .4 1 1 1 97.C -84 .7 6 13 1 - 2 . 2 I. 1 -3 2 62.4 -65.9 -5 1 1 - 4.7 - 3.C 11 ft 12 t 14.9 - -2.2 14.5 -1.2 ~2 5 1 13.7 t 21 .3 16.4 2C.6 -6 13 7 13 1 -2.2 1 13.8 7 1 -13.9 4 -4 2 38.5 2 27.4 37.5 31.4 -6 1 1 44 .C 1 B4 . 1 4C.9 PC.6 t i £ 7.9 -7.9 1 47.C -49.1 -7 1 ! 1 -7.3 C .4 5 2 -1.8 -C.9 1 79.2 -7?.5 14 « 19 6 I - 2 ; 15.1 4.8 11.9 - 3 \ L 1C4.9 1 32.1 ICC.4 -35.6 8 t ; -a 13 t 9.1 1 1C.7 -».« -8.6 -3 6 \ 2 2C . 4 2 4 3 . 3 18.8 4C.0 B t 3 41.7 1 41.1 -41. J -41.9 C 8 9.1 -5.9 4 5 1 1C.3 -8.3 9 13 1 13.1 13.2 -6 2 -t.e 1.7 -8 I 1 34.2 - 5 1 . 2 1 a -1 .7 -1.7 I 5ft.9 59.7 • -9 13 1 - 2 . 3 - 1 . 3 7 2 2e.4 25.2 9 1 1 35.1 55.1 2 e c IC. J - 1 C . 5 9 5 I 3 3 . 3 -3C.C 10 13 1 -2.1 2.1 -7 t 2 9 . 9 -10.5 -9 1 3 38 . 2 17 . 2 3 e 7.2 t 14.C 14.9 ' -10 13 1 11.4 ' l l . B a 2 24.4 -22.1 to 3 34.4 37. 1 4 e 9 a 0 34.e - i . e 32.8 1.4 -t 1 1 19.1 I 46.5 -17.5 -44.6 0 19 1 15 1 I C C 1 15.5 -9.4 • 11.8 -8 9 I 2 -2.C 2 -2.1 4.6 -1.7 -to 1 11 1 3 14.5 3 21.4 34 .9 -21 . B a a T a 0 e 9.ft -2 .C - i c i A . 3 -I 1 1 33.2 1 32.8 33.6 -32.1 -1 15 2 15 1 U.7 1 12.4 -17.fi 11.6 - 9 10 I 2 26.4 2 17.4 27.fi 17.6 - t l 1 12 1 1 76. e 3 - 2 . 2 -77.8. C.C a a 0 2 i . 2 2 2 . 3 o •> 1 5.3 10.7 -2 15 t 7.4 8.1 -10 * 2 S.C -8.3 -12 1 3 24 .5 - 2 6 . 2 9 e c ice -7.9 1 41.t 41.3 3 19 1 13. a -11.9 ' 11 2 te.c -16.4 1 1 1 1 2 1 . 2 18.9 10 a 11 a c 0 •2.2 -2.2 -5 .2 -3.9 I 35 . 2 1 29.2 - 3 5 . 3 27.4 - 3 t3 4 15 1 18.5 I -2.3 IB.9 1.4 -11 12 2 24.8 2 -17 . 3 -24.1 -15.9 -11 1 14 1 1 15.4 3 -2.4 14 . 4 -7.1 12 a 13 a 0 c -2.2 -2 . 4 -ft.9 -4.C -10 1 1 7.4 1 33.1 8 . 3 -29.8 -4 15 5 15 1 I C S 1 15.ft -8.8 16.7 -17 13 \ 2 - 2 . 2 2 -2.5 -2.0 1.6 -14 1 15 1 1 1 l.t 3 7 C 4 1C.6 -19.1 14 a c -2.? -2.5 It 5 I 17.1 15. 2 -5 13 1 12.1 -1C.9 - t i 6 2 21.1 18.5 -15" I 1 - 2 . 4 - 7 . 4 c 1C c -2.C -5 .4 1 -2.2 l.A 6 IS 1 -2.1 -2.9 14 2 13.1 14.2 -16 I 3 B.7 -H.fc 1 1C 2 1C c c (.9 -J.C 4.9 3.5 -12 « i a.7 t 21.e -25.2 19.9 — ft 15 0 C 1 1C.3 2 21.4 I C C -21.5 -14 15 2 -2.4 2 -2.1 -7.1 0.1 0 3 1 1 1 4 7.8 1 l.t -44.H 5. 7 3 1C c c -2.C 22.1 C.4 -21.C l 12.8 1 - 2 .2 -11 .9 - 2 . 9 1 c - i e 2 2C.ft 2 47.9 18.fl 47.9 -15 0 ; 2 12.C 2 -1.8 -11.6 1.7 -I 3 2 1 1 5.C 78.9 3.7 75.5 9 1C 0 -2.1 i.a 14 3 1 19.ft 16.4 7 c 2 81.C 81.9 1 8 2 6.4 6.1 -3 3 I 4 4 . 4 «A . t A IC c 13.C 13.1 I 14.7 -14.5 - 2 C 2 Tl.ft 72 7 -I 2 5.ft 4.4 1 ; 3 35 .8 -11.5 7 1C 0 ft.9 8 . 9 15 5 I 13. ft 12.3 7 C 6ft.7 -55.1 2 g 2 14.ft 12.1 - 3 1 1 4.7 4.1 • IC c -2.2 -5.8 -13 5 1 - 2 . 4 5.5 - 3 C 2 89 . 4 -90 . 1 -2 B 2 2C. 1 19.4 4 1 1 61 . 2 - 6 C . 5 ' 9 tC 10 IC 0 C 15. e -2.2 -13.7 -T.7 -IS I 1 7 .9 1 12.1 -7 .1 U . C 4 C - 4 0 2 94.9 2 I5.C -111 . 3 -14.ft 3 - 3 B e 2 6.4 2 2 C 2 7.1 -23.9 -4 ; 5 1 1 61.7 1 6 C 6 -62.C 61.1 11 IC a .5 1 . 3 0 1 1 -I.J - 4 . 4 5 C 2 27.4 -75.6 4 « 2 -1.9 -4 8 -4 3 3 15.fi 13.5 12 IC 13 IC c c i i . e -2.2 11.6 ft.7 -1 I i 27 . e 1 1C.9 -24 .4 9.3 -5 C 6 C 2 6 C 5 2 11I.C 60.8 104.9 -4 3 8 8 2 9.3 2 5 . 3 -10.4 -8.6 -6 1 3 29.5 J 54.2 25.4 55.4 0 12 c 16.3 -17.9 2 1 1 7.1 - 6 . 4 -6 C 2 2C.3 -19.9 -3 B 2 17.5 19 . 2 7 1 1 5 2 . 2 -51 .1 1 12 2 13 c c - 2 .2 2C.9 2.4 19.4 'I i 1 19.2 i 4 c . e 70.1 17.7 - 7 C 68.2 2 91.t 64.2 -86.5 6 -6 B 8 3 -23.C 2 e.i 22.5 -7.6 -7 3 8 1 3 14 . 3 3 14.7 -14.9 -17.C 3 12 c 15. ft -15.3 -3 7 I 36.e -36.5 8 C 2 64. C -64.6 7 8 . 2 - 2 . 1 a.e J 55.! -*8.4 c 16.4 - 1 5 . 1 l 25.9 24.2 2 -1.9 1.5 -7 e 2 i c . i -6.5 9 1 3 5.4 71.5 9 12 A 12 c c -2 .2 - 2 .2 4.9 3.0 , "5 J I 45.4 1 l i . 8 46.7 -14.0 -I I 22 57.8 -7.4 51.7 B -B 8 . 8 2 t l . 5 2 -2.1 - I C l 5.6 - 9 1 10 3 1 25.C 3 -2.7 24.4 -1.1 7 12 a 12 e c -2.2 1 1 .ft 9.C -12.5 'I ; 1 23.1 1 11.7 24.4 9.T -IS I 2 7 3 . 3 2 -2.7 70.1 -0.4 9 -9 8 e . 1 -3.2 2 -2.2 - 1 . 3 -1.7 -tc 1 11 3 3 4« .5 3 18.7 45.8 -71.3 9 12 c -2 . 4 2.2 —A 7 1 37.1 - 3 5 . 9 11 C 2 -2.1 -0.7 10 8 2 136.9 7.7 -11 1 1 IS.3 -14.9 10 12 c 13.3 8.5 7 7 1 1 3 . 3 10.4 -1 1 c 2 4 9 . 2 -41.9 -10 8 14.ft — 1 4. 3 12 3 1 13.7 -14.1 11 i i C 14 c c -2.2 15.e - 5 . t -12.1 'I J 1 12.8 1 -2 .C -12.1 - 4 . 0 -12 I 2 41. t 2 24.2 -45.6 24.7 11 -11 a ~ e 7 7.C 2 8.7 -4.8 - f l . 3 -12 3 13 3 3 1(5. 1 1 76.1 -I5.fi 77.7 t 14 c -2.2 2.8 ' -6 7 1 26.7 27 .4 13 C 2 - 2 . 2 1.6 12 9 2 -2.4 -6.7 -13 1 1 1 1 .2 16.C 2 14 c it. e 17.4 9 7 1 18.9 -18.1 -13 C 2 4ft.t 44.A -12 a 2 -2.2 - 5 . 1 14 ; 3 - 2 . 4 4.fi 3 14 0 i.t -7.4 -9 7 1 -2.1 -2.7. 14 C 2 17.2 14.9 11 a 2 . -2.1 4.6 -14 3 3 1C.3 A.9 4 14 c -15.1 1 8.5 7.5 -14 C 2 3i.i - II a -13 8 2 7.4 8.5 15 3 1 2 C C -70.4 9 14 A 14 c c B.e 12.4 7.2 12-8 " u ! 1 17.8 1 12.2 -16.2 13.7 15 C -15 C 1 15.i 2 22.5 -13.9 -25.4 14 - 14 B a 2 7.5 2 -2.1 7.4 5.C -15 1 -16 I >. 15.9 3 -2.2 -17.1 -2.6 7 14 0 -2.2 -e.i - l l 7 1 - 2 . 2 -3 . a 16 C 2 9.E -6.8 0 " i c 2 - 2 . C -0.1 0 . 5 3 7 2 . 4 -72.3 a M c -2.2 7 4 12 7 1 ice -8.3 -16 C - 2 . 3 4 . 4 - 1 IC 2 -2.1 . 1.3 1 3 1 8.8 - 5 . B c i t c 11.5 -13.2 -12 7 1 -2.2 -A.a -17 C 2 12.5 11.1 . -I tc 1 -7.C - 5 2 -1 5 3 27.3 -21.7 c -2.2 2.2 1 11.C -10.6 2 11.4 8.C 2 w 2 1C.3 -9.3 2 5 15 ft 20.8 2 1* 3 IC c c ie.i - 2 . 1 17.0 -1 .0 1 -2.2 I - 2 . 3 5 .4 3.1 -1 Z 1 2 85.5 -Si.7" ' 94.4 -2 3 ic tc 792 - 2 . 1 79 -1.6 -2 5 3 5 3 79.8 3 6.5 11.7 4.7 - 23 -Table VII - cont. Continued :-h k I F0 Fc -3) 3 3 24.e 24.1 4 3 ) 37.9 -31.4 -4 9 3 28.4 -29.8 5 9 3 38.A 34.9 -9 9 ) 4.2 7.3 4 9 3 14.1 13 .3 -6 9 3 t l . C 16.3 7 9 3 34.9 -32.1 -7 8 3 fr.l 0.1 8 9 3 2C.8 -20.a -8 9 ) 7.8 -5.3 9 9 3 28.3 26.3 -4 9 ) 13.J 16. 5 10 9 3 12.1 12.3 -10 3 ) 28.4 28.6 11 5 3 27.4 -25.2 -11 3 3 23.3 -23 .9 12 9 3 -2.2 -1.0 -12 3 3 24.3 -32.B i) s 3 i s . i 13.a -13 3 3 14.9 12.7 14 3 ) -2.3 -2.C -14 3 3 11.3 12.3 -IS 3 3 12.4 -11.9 0 T ) 24.C -25.1 1 7 ) -1.8 t.O -I » 3 22.1 -22.2 2 3 ) 31.6 39.1 -2 7 ) U.4 12.1 3 » 3 -1.9 -3^2 -3 7 3 -1.8 -0.4 • 7 ) IS.* -14.4 -4 7 ) IC.7 -11.4 9 7 ) 19.9 19.6 -9 3 ) 10.9 -8.6 6 7 3 18.2 13.7 -4 7 ) 11.9 11.9 T 7 3 11.1 -9.5 -7 7 ) -2.1 -3.3 * 7 3 7.7 -6.3 - 8 . 7 3 18.5 -20.1 9 7 3 11.1 9.3 -9 7 3 11.1 12.5 10 7 ) 8.1 7.9 -10 7 ) 7.1 6.5 11 7 3 18.9 -16.8 •11 7 ) 14.2 -12.1 12 T ) -2.4 2.7 -12 T 3 9.1 -9.5. 13 T 3 a.! 9.0 -13 7 ) -2.4 5.5 -14 7 3 -2.3 6.2 0 9 3 -2.C -2.7 t V 3 -2.1 -1.3 - 1 9 1 -2.C -0.5 2 9 ) -2.1 -1.3 -2 9 3 14.8 16.2 3 9 1 -2.1 -3.5 - 3 9 ) -2.C 6.2 4 9 3 6.7 6.2 -± 9 3 13.1 -1C.2 5 9 ) -2.2 -4.0 -9 9 ) -2.1 -0.9 6 9 3 8.3 6.7 -6 9 3 -2.1 -7.B 7 9 3 -2.2 4.9 -7 9 3 -2.2 -5.6 9 9 3 7.9 -7.7 -8 9 3 -2.2 -3.8 9 9 1 -2.2 3.8 -9 9 3 -2.2 2.3 10 9 J -2-4 0.5 -10 9 ) -2.2 0.4 11 9 ) -2.3 -3.0 -11 9 1 -2.5 3.6 12 9 ) -2.2 2.2 -12 9 3 -2.4 1.3 -13 9 3 -2.1 -1.4 0 11 1 -2.2 -4.2 1 11 3 -2.2 • -2.1 -1 11 3 4.2 1C.3 2 U 3 24.? -25.2 -2 It 3 13.< 14.7 3 11 3 -2.2 O.T -3 11 i «.3 9.2 4 11 3 7.1 8.C -4 t l 3 8-5 7.4 9 t l 3 12.7 -12.2 - 5 11 3 -2.2 -1.4 6 11 3 -2.2 -t.3 -6 11 1 13.i -13.1 T 11 3 10.4 8.8 —T 1 1 3 -2.3 -1.6 8 11 3 -2.4 -2.1 -8 11 1 12-9 15.1 9 11 3 -2.1 -5.1 -9 11 3 1.1 -8.5 10 11 3 -2.2 2.6 -10 11 1 -2.4 -C.7 -11 11 3 8.6 8.1 0 13 3 16.1 12.3 1 13 3 -2.2 0.4 -1 13 ) -2.2 7.1 2 13 3 -2.2 -7.1 -2 13 3 17.4 -13.1 3 13 3 -2.'. 2.4 -3 13 3 -2.2 - l . l * 13 1 7.6 9.1 -4 13 1 14.1 11.8 9 13 ) 9.2 -9.8 -9 13 3 -2.4 -4.3 6 13 ) 8.9 -8.4 - 6 13 ) 14.1 -12.9 7 13 3 9.3 10.5 -T 15 3 -!.3 1.6 -B i ) 3 a.e 9.3 0 IS 3 K.4 12.2 1 15 3 11.9 -9.3 - I 15 3 -2.2 -0.7 2 15 3 13.5 -12.1 -2 15 3 io.a -11.B -3 15 3 -2.1 3.2 0 C i - t . e -1.4 - 1 0 * 42 . ) 43.2 -I 0 1 31.9 -32.9 2 c * 6.3 -5 .7 -2 c » 2C.I 18.8 3 0 % 81.2 -75.9 -3 0 k 62.7 76.T 4. 0 4 3C.1 -30.6 -4 c » 31.1 -30.6 3 0 * 60.5 38.3 -5 c I TC".e -U . I 6 0 * - 1 . 9 - 3 . T - 6 0 ti 61.7 38.9 7 0 k 41 r 5 -43.5 -7 c t 31.1 30.6 8 a k 66.9 62.a - 8 0 94.9 -36.1 9 c 9.6 1C.2 -9 c 92.3 -53.6 10 c t 3 3 . t -13.7 -to a k t l . C 13.8 11 c k -2.2 -4.5 -11 c 29.1 30.3 12 c k 28.7 27.9 -12 0 -2 .9 -4.4 13 a 12.3 IC.6 -13 c -2.3 2.4 14 c 14.5 -14.8 -14 o k 13.4 14.3 -13 c -2.3 1.7 . 0 2 24.6 -24.C 1 2 33.6 56.5 -1 2 91.3 -34.7 2 2 t.C 4.4 -2 2 21.C 21.0 3 2 61.2 -62.0 -3 2 46.1 47.2 4 2 19.1 17.9 -4 2 13.4 -16.4 2 It.8 41.7 -5 2 49.C -48.3 6 2 33.1 -13.3 -6 2 32.e 31.2 7 2 27.8 -32.1 -7 2 42.7 40.4 B 2 40.8 40. C -8 2 41.4 -19.7 9 31.ft 30.1 -9 2 30.4 -27.2 10 2 23.7 -21.2 -10 2 32.1 13.5 It 2 ta.e -19.9 -11 7 1G.0 18.6 12 2 " t l . C tO.2 -12 2 4 18. t -20.0 1) 2 T.! 10.5 -1) -2.S -1 .9 14 2 16.6 -16.7 -14 2 < i s . e 13.6 -13 2 -2.3 0 . 8 0 11.C 10 .t 1 4 67.3 63.3 -1 4 37.1 -57.3 2 6 c c -8 .1 -2 4 -1.1 9.B 3 4 4C.1 -40.1 -3 4 3C.3 )2 .C 4 4 16.4 19.9 -4 I C C -11.8 9 4 35.9 27.3 -3 4 • 11.6 -17.7 6 4 21.5 -21.C - 6 4 29.2 30.9 7 4 2 7 . * -25.C -? 3C.9 32.3 B 4 It.9 9.1 # -6 4 -2.1 -20.9 4 36.7 33.3 -9 4 ' 16.4 -15.2 # io 4 e . i -25.6 -Ifl 3*.T 24.C * It 4 i c e -24.3 -11 -2.2 3.9 12 4 13.9 14.1 -12 4 22.7 -23.2 13 4 8.1 9.1 - U -2 .5 -6 .7 -14 * 2C.4 20.3 -15 4 -2.2 -0 .6 0 6 -1 .9 -4.C 1 6 30.8 30.1 -1 6 37.7 -38.4 2 8.1 6.4 - I -1.4 -1 .3 3 t 22.1 -2C.C -3 ( 33.8 35.9 4 ft -2 .C -2.3 -4 6 17.1 -16.2 5 12.3 13.C -5 ft 22.6 -22-9 ft k -2.1 -0.1 - 6 k 2C.1 21.2 7 6 8.5 -9 .C -7 6 22.e 22 .9 1 7.S 4.1 -8 « 12.4 -15.1 9 6 11.2 9.1 -9 6 14.C -16.3 10 6 k 17.9 -17 . C -10 t 10.C 7.B 11 16. 4 -15.7 -11 t -2.2 2.5 12 6 • 17.6 17.6 -12 6 k 8.8 -9 .7 13 e k 8.3 7.0 -1) t > -2.4 - 3 .6 -14 6 12.1 11.9 0 8 k 11.4 -12.3 1 8 k -2.1 5.2 -1 • 24.4 -27.C 2 6 18.1 18.8 -2 a k e.T -7.2 3 B -2.1 -7 .5 -3 a 8 .7 4.9 4 a k -2.2 3.9 -4 a -2.1 -3.6 3 a 1.8 7 .9 -5 8 . k 9.5 -12.6 • a 4 -2.2 -4.9 -4 6 4 -2.2 -0.8 7 8 4 -2.2 0 .9 -7 8 4 12.2 14.0 B t 4 1.9 7.1 -a 8 4 8.7 .-8.2 9 8 4 -2.2 3.4 •9 8 4 -2.2 -0 .9 10 a 4 -2.4 -0.2 -10 8 4 -2.2 8.3 4 -2.3 -»;r -11 t 4 -2.4 3 . ) 4 -2.) - 9 . 8 - 1 3 8 4 -2.2 - 0 . 9 0 IC 4 27.3 24 .1 i i c 4 14.1 13.9 - i to 4 -2.2 3.7 l to 4 14.1 -11.2 - 2 10 4 -2.2 - 6 . 8 3 10 4 -2.2 -4 .1 - 3 tC 4 16.1 -16.7 4 10 4 7.1 -7 . 3 -4 10 4 -2.2 -4.1 9 IC 4 -2.2 -0.2 -5 10 4 17.5 17 .3 6 10 4 -2.2 3.8 -6 10 4 -2.2 4.4 7 10 4 -2.5 -6 . 6 -7 10 4 9.8 -7.4 8 10 4 9.3 -8.1 - 8 IC 4 -2.2 3.9 9 10 4 -2.3 3.0 -9 10 4 -2.4 -t.« 10 IC 4 -2.1 4.9 -10 10 4 -2.1 -2.8 -11 IC 4 -2.2 1.0 0 12 4 -2.2 3.8 t 12 4 -2.2 9 . B - t 12 4 It.4 13.1 2 12 4 -2.2 - 9 . 9 -2 12 * -2.2 -0.4 3 12 4 -2.4 3.3 -3 12 4 I C C -13.5 4 12 4 -2.4 -2 . 8 -4 12 4 -2.3 5.0 9 12 4 12;* -1C.9 -5 12 4 ,,16.4 17.9 6 12 4 -2.3 2.4 - 6 12 4 -2.4 -4.a 7 12 4 -2.2 ' 4.4 -1 12 4 13.3 -11.0 '-8 12 4 8.1 4.3 -9 12 4 -2.1 - c i "" 0 ' 14 4 -2.2 -2.3 1 14 4 15.1 -12.9 -1 14 4 9.S IC.) 2 14 4 -2.2 3.2 -2 14 4 -2.2 -).4 3 14 4 12.3 11.0 -3 14 4 11.3 - t l . 6 -4 14 4 -2.1 4.1 0 . 1 5 41.1 19.6 1 1 3 IS .9 30.4 -1 t 1 11.5 -12 .7 1 4J.51 -41.6 -2 1 3 42.6 -43.6 * ) 1 3 i i . e -29.4 9 28.3 28. C 4 1 3 33.8 37.2 -4 1 5 29.6 31.4 i a.1 J . l -5 1 3 58.1 -15.9 5 44.3 -41 .6 - 6 1 3 36.2 -17.0 7 1 3 -2.2 *2.4 * -1 1 5 -2.4 4C.1 3 3t.< 37.0 - 8 t s ie.7 16.« 9 1 9 18.8 "-18.4 -9 1 3 29.2 -28.3 10 1 5 17.1 -14.8 -10 I 3 -2.3 -4.0 3 J.4.4 24.3 3 -2.! 30.4 12 1 9 18. t 18.9 -12 1 3 -2.9 -1.1 13 1 3 17.9 -15.8 -13 t 3 18.1 -11.4 5 -2.3 4.1 0 3 5 42.2 40.8 I 3 3 12.7 14.3 -I 3 3 2ft. / -21.2 3 46.? -12.8 -2 3 5 22.7 -22.C 5 9.C -9.1 -3 3 3 33.1 32 .6 4 3 5 41.4 43.3 -4 3 9 41.1 43.3 9 ] 3 14.2 I t . ) -5 1 3 15.1 -33.4 4 33.5 -32.9 3 19.8 -18.4 3 -2.2 3.1 -7 3 3 31.8 31 .1 . 0 3 5 8.7 16.9 - 8 3 5 13. C 12.5 9 3 5 -2.2 -4.8 -9 ) 3 22.! -21.0 10 ) 3 14.C -23.1 -10 ) 5 -2.5 -0.1 11 3 5 12.6 13.1 - I t 3 5 11.1 16.5 12 3 3 Id. 5 t * . l -12 3 9 -2.3 -6.9 -13 3 9 t e . i -20.6 -14 3 9 -2 .2 1.4 0 9 5 3C.1 32.1 1 S 5 -2.1 .3.3 3 19.9 -18.7 2 3 5 16.8 -16.5 -2 3 3 32.C -32.6 3 9 5 -2.1 6.3 -3 3 5 If.ft 39.1 4 S 5 28.4 26.7 -4 5 9 16.2 13.6 5 5 9 -2.2 1.S -5 "5 5 29.ft -30.2. * . 5 3 21.S -24 .3 5 I C 1 -11.) 3 - 2 .2 - 2 .2 9 23.6 21.0 9 19.1 21.C S 1.1 7.6 3 12.1 - U . 6 9 12.8 -12.* 3 23.C -22.4 -11 5 -2.2 0.7 3 -2.1 9.1 -1 5 - 2 .2 9.4 3 7.3 B .3 - i : 5 -2.4 0.8 -13 5 16.C -14.8 7 - 2 .2 t.C 7 - 2 . 2 1.) 7 23.1 -22.4 7 11.4 -17.6 7 9.C -9.3 7 -2.2 -1 . 6 T 2 C 7 19.4 ? 18.9 20.1 1 -2 .2 -4 ,9 J - 2 .2 -4 . 3 7 1.1 -8.3 T ) . l -7.2 1 13.2 -11.8 T - 2 .2 . 4.1 1 12.1 11.3 7 -2.1 6.6 7 12.3 14.2 1 -2.4 -1.3 7 t.t -8.0 T -r2.1 -4.5 - t l 7 -2.5 - l . t 7 -2.1 0.8 1 .5.2 7.4 -1; 7 -2 .2 -3.9 9 -2 .2 -1 .3 9 •-2.2 -4.S 9 -2.2 -2.3 9 18.4 -13.6 9 11.) T.e ' 9 - 2 .2 -S .8 9 - 2 .2 -2.4 9 13.2 It.9 9 - 2 .2 1.6 9 - 2 .2 1.5 9 -2.2 t.e 9 -2.4 -2.7 9 -2 .2 - C B 9 -2.4 3.1 9 -2 .2 0.4 ' 9 -2.3 -3 .9 9 -3.4 0.3 9 -2 .2 1.8 9 -2.4 -4.2 -IC 9' -2.3 - l . C . -1 9 -2.1 5.8 11 -2.1 -1.5 11 -J.S -3.6 11 15. 5 16. 1 11 -2.4 -2 .4 11 13.5 12.6 11 -2.4 2.4 It -2.5 -5.1 11 -S.4 0.5 t l -2.4 -1.1 11 - 2 . 3 1.1 11 -2.4 4.7 11 J - 2 .2 3.8 11 1.4 6.6 11 i.i -6.1 II 5 9.6 -9.3 It - 2 .2 -6.4 13 9.1 -9.1 13 S -2.1 -6.1 13 i 8.4 6.6 13 -2.1 3.2 13 5 12.B 14.4 13 » -2 .1 -6 .0 C 31.3 30.0 ' c 4C.9 -38.6 c 1 22.5 24.4 S 3S. 22.7 -21.5 c t> 19.4 -16.3 c t -2.3 2.9 -1 J 0 6 18 4 -15.C 6 14.5 14.3 6 2C.4 21.0 - j c 6 22.4 • 21.0 » 6.9 -8.3 2 b • 17.2 11.1 2 ft 11.1 -10.4 2 6 23.2 26.3 2 6 14.3 -10.1 2 6 13.4 -32.6 i 2 6 2E.1 26 .6 i 2 » 17.4 -17.4 k 2 b 14.c 11.4 k 2 6 42.1 40.8 2 t e.i -19.2 2 a i.e 7.2 2 6 9.4 -14.3 2 6 21.8 -21.6 * t 9.4 20. t 2 6 -2.5 0.2 i 2 6 - 2 .2 1.5 I 2 6 21.C 22.0 9 2 6 18.3 -18.4 6 9.1 -10.1 Q 2 6 -2 .1 1.8 -1 1 2 6 22 .7 -25.2 2 6 1B.1 18.1 - t l 2 A 7.C 7.3 -12 6 t i . e 1ft.1 -13 ; 6 -2.1 -5.4 6 21.9 i i . i 1 4 4 4.4 -3.9 -1 4 6 14.2 13.7 2 4 6 -2.2 -4.4 -2 4 6 )6.2 -34.1 ) 4 6 15.1 13.T -3 4 6 12.1 - I t . ) 4 4 « 14.5 14.4 -4 4 6 41.ft 41.1 9 4 6 21.8 -14.4 -3 4 6 -2.2 -0.3 6 4 6 15.8 -13.4 -6 4 6 25.1 -24.1 T 4 6 29.3 27.2 -1 4 6 -2.2 -0.4 • 4 6 -2.4 2.3 4 6 22.4 22.0 4 4 6 11.7 -17.6 -9 4 6 -2.2 -3.1 10 4 * -2.2 0.3 -tO 4 ft 13.9 -15.7 -11 ' 6 -2.3 -1.2 -12 4 4 12.e 11.1 6 -2.2 5.4 I 6 ft 8.1 -6.7 -I i ft -2.2 0.1 7 ft 4 -7.2 -) .a -2 ft 6 23.ft -26.8 1 ft 4 2CC 17.8 -3 ft ft -2.2 -3.1 4 6 4 14.( IB.8 -4 ft 6 11.e 11.7 5 6 6' 24.8 -26.2 -5 4 6 I C C 10.6 6 ft 6 -2.1 -5.2 -6 6 6 13.1 -12.9 7 6 6 17.C 17.1 -7 6 6 -2.2 0.) 8 6 6 -2.3 4.6 -B 6 A IC.4 11.6 9 6 6 1C.4 -10.1 4 -2.4 -C.4 -10 ft 6 9.C - t . l - 11 ft 6 -1.2 4.3 ft I C C 9.A | 1 6 -2.2 -1.5 -1 1 6 -2.2 -4.4 6 i i . : -12.5 -2 1 6 -2.i -2.9 1 1 ft 12.5 12.2 -3 0 6 -2.2 2.6 6 -2.4 t.4 -4 1 6 -2.2 -1.3 6 U . C -15 . i A ft.9 4.4 A i 6 -2.1 C. 1 -6 1 ft -2.3 - C I 7 a ft -2.2 2.4 - 7 6 . 6 -2.4 -1.6 6 -2.1 0.6 ' -8 i 6 1.8 9.4 -9 a 6 -2.2 -0.1 ft 8.9 -4.C 0 11 6 -2.4 ?.b 1 IC ft 12.4 10.1 - I 10 6 -1.4 -5.6 6 8.2 3.4 -2 11 6 -2.4 0.7 3 IC 6 -2.3 -3.1 - J K 6 -2.4 C.6 4 IC A i.e - l . t ft -2.3 a.3 3 IC 6 -2.1 -0.2 -5 IC 6 -2.3 -1.9 -b 11 6 -2.2 -C.J -7 IC 6 -2.2 -2. 7 1 4.4 - U.9 7 42.1 -19.1 7 4(.8 44.1 2 7 I C C 9.6 -2 7 12.8 11 .9 * ) 7 -2.2 18.1 - ) 7 32.C -10.2 4 1 7 IC.5 -15.9 *4 7 -2.1 1.1 9 7 2 C * -21-4 -9 7 15.1 16.1 a 7 12. C 11.2 -6 7 15.1 -14.«; 7 7 l t . 1 15.3 7 1.5 -8.2 a 1 12.* -11.6 -a 7 7.1 7.5 -9 7 11.2 16.2 - IC i e.e -8.4 -11 7 8.9 -1C.6 7 -2.2 -0.4 1 19.1 -1B.1 _ 1 7 21.1 27.8 .7 14.5 11. e -2 1 -2.2 C.4 3 7 20.1 20.4 - j 1 26.C -26.1 4 7 14.C -16.A -4 1 -2.2 5.2 9 7 12. L -9.6 -5 1 IS.5 11.1 6 7 -2.4 12.1 -6 7 -2.2 -6.4 7 7 13.1 13.ft _ 7 7 2C.< -22.6 • 8 7 14.C 1 12.C IC.9 -9 7 i t.e 10.C -10 1 -2.2 -11. 7 7 I C 5 -9.1 1 7 18.C -16.1 -1 ' 7 K . I 9. ft 2 7 -2.5 3.6 .2 7 -2.2 6.4 ] 1 21.1 19. 1 -1 7 12.4 -12.8 4 i . 1 -2.4 0,4 -4 S 7 -2.2 - I .9 5 7 12.2 - 12.6 - 24 Table VII - cont. C 12.2 - 1 3 . 9 Y 1 Fo'Fc 15.1 16 .1 IC.7 11.7 8 .6 - 9 . 1 8 .3 9.2 11 .5 - 1 4 . 9 0 -2.2 - 3 . 9 C 18.1 1 7 . 8 0 -2.2 - 0 . 4 0 3 4 . T -36.7 0 27.t 2 3 . 5 0 6 4 . 1 6 8 . 4 0 2 C . 9 - 2 1 . 4 0 5 9 . 4 - 6 C . C 0 2 4 . 4 3 1 . 4 0 2 t . 9 2 7 . 9 0 I C . l - 4 1 . 8 Q 2 2 . 6 - 2 0 . 5 0 4 . 3 4 . 9 C 1 7 . 6 1 6 . 6 C 1 7 . 4 - 1 7 . 5 0 -2 . 3 -8 . 6 16.7 1 7 . C 1 3 . 4 14.7 -2 . 4 -7.8 7.9 -8.7 1C.1 8.7 -2 . 3 . 1.0 -2.1 7.2 7.6 -7 . 4 -2.2 - 4 . 3 -7 .4 -3.2 -2 . 3 - 9 . 1 1.4 7 .9 -2 . 3 0.1 -2.2 -3.1 -2.2 2 .6 -2.2 -1.1 1 0 *7 .5 -58.7 C 2 4 . 4 22 .4 0 2 9 . 3 2 8 . 8 C 21.2 - 2 0 . 2 0 2 9 . C - 2 5 . 6 C 2 C . t 1 9 . 7 0 18 .6 2 0 . 7 0 14 .1 - | 4 . 1 0 2 3 . t -22 .6 0 1 7 . 9 U.2 0 19.2 -19.7 C 3 3 . 1 - 3 6 . C -2.2 l . B - 3 . 1 - 4 . 4 -2.2 - 2 . B -2.2 -0 . 8 -7.1 U C 17.9 - I t . 6 C -2.3 -1.3 C 2 5 . C 22 .8 0 -2.2 -6 .1 0 1 6 . 4 -17.1 0 -2 . 3 8.C C . 14.7 2 0 . 9 -2.1 - 1 . 9 -2 . 4 7.1 2 1 . 3 1 8 . 8 13 .6 1 5 . 6 6 .8 - 1 C . 4 11.C - I t . 4 6 -2.4 - i . C 0 7.2 -8.1 C 1 1 . 7 17.B 0 1 3 . t -16.7 0 -2 . 4 - 4 . 9 0 1 6 . 6 16.1 11 .7 -2C.7 9.8 - 1 0 . 1 1C .C 9 .4 77.9 22.ft 14.1 12 .C 8.5 -fl.2 t G -2.1 0 .5 11.2 - 1 1 . 6 -2.2 2 . 8 29 .1 -31.9 6.1 8.1 44.1 104.5 21.* -22 .8 - 2 . 3 0 . 6 1 -7 . 4 3 .3 75.9 2 1 . 9 12 .4 1 5 . 7 - 2 . 2 - 7 . 4 125.C -IU.1 1 1 3 . 1 9 6 . C 1 3 . 1 - 1 3 . 1 1 0 1 . 1 - 1 0 4 . 2 3 1 . C 31.n 2 9 . 4 ? T . 5 9.1 - 9 . 6 10 .1 - 1 7 . 4 11 .6 - t l . l 12 .3 1 2 . 4 11.7 9.1 1 -2.2 -11.7 12.1 10.fl 7 3 . C 69.1 I t . 4 - 1 6 . 1 11 .1 17 .1 8 .9 5.9 2t.1 -27.7 k k 3 17.•! - 1 7 . 6 » -2.2 2 . 0 1 -2.1 -0 . 9 1 18.1 19.2 i i>.c ii.a 9 -2.1 2.T 3 5 . 6 - 3 4 . 5 . 23.e - 2 1 . 9 1 2 . 9 1 1 . 3 15 .e -12 . 1 . 22.ft 21 .1 1 3 . t 1 1 . 9 k 8 -2.! -5.2 k . 8 I I . T -12.2 8 t .1 1 .5 k e 9.5 i a . i l O 29 .B - 3 0 . 4 C 12.2 -7.2 3 3 . 4 -Jl . 5 1 6 . 1 - 1 3 . 5 24.ft - 2 2 . 1 -2 . 4 4.C 12.f 12 .C 1 1 . C . 1 6 . 8 I C C 9 . 4 -2 . 9 6 . 6 -2 . 4 -5.1 -2 .5 - 6 . 6 L C 13 . J 1 0 . 9 C . 6 1 . l ' - 6 2 . 4 I C 8 .3 4 . 4 1 0 4 4 . 8 -39.2 I C - 1 . 4 O.b C 14.3 - 1 2 . 5 C 14.7 1 3 . 4 I 0 29 .1 20 .G 1 C 11 .C -7 . 3 I C 8.4 - 3 . 3 t c e.i o . 4 1 C 7.7 - 5 . 9 I C -2 . 4 - 4 . 5 1 0 -2.1 2 .6 3 0 17 .8 - 1 9 . 8 J C 24.7 - 2 8 . 6 -2 . 4 -2 . 6 -2 .1 C I 3 t . l - 5 2 . 5 3 6 . 4 - 5 4 . C fcC.2 - 5 B . 4 2 4 . 5 2 8 . 8 8 5 . C 87.4 1 8 . 7 1 7 . 8 5.2 -O . B 1 8 . C - I t . * 3 9 . 3 - t l . 9 - 1 . 4 - 4 . 1 3 C 53 .1 5 1 . 9 3 C 9.C - 9 . C 3 C 4 2 . C - 3 9 . 9 J C - 1 . 4 3.1 1 C 24 .C 1 0 . 4 i C 17.7 - 1 6 . 9 1 9 . 6 T 9 . 6 6 1 . 3 60.1 24 .1 22 .1 9 .1 - I C * ice - 5 0 . 1 16 .C - 1 5 . 4 ! C 18 .4 -17.a * C 17 .4 1 5 . 4 9 0 11.1 9 .4 J 0 22.2 - 1 4 . 6 3 0 11.2 -11.7 1 C 8 .7 (l.t. 2 1 . 5 - 1 9 . 9 11.1 16.1 4 C . I 42.2 2 8 . 3 2 8 . 3 11 .8 - 1 0 . C 1 2 . 2 - 1 5 . 9 I C - 2 . - 6 . 3 3 0 1C .9 - 1 0 . ? 1 0 18 .8 -39.1 5 C -1.1 - O . C 3 0 48.8 9 0 . 6 J 0 7.C 7 .6 -e.e - t o . ! 2 3 . 8 -2B.1 -2 . 5 3.1 I -2.2 0 . 4 1 1 1 . 9 B . l 1 2 . t 11 . H 1 C 55 .4 - S 4 . 4 5 0 51.9 4 7 . C I 0 32.2 4 9 . 1 9 0 12 .1 - 3 2 . 6 9 C 15 .1 - 3 3 . 9 S C 4 6 . 3 4 4 . 2 1 -2 . 5 3 .5 I 9.2 - 1 . 8 1 1 1 . 3 - 1 4 . 9 1 6 . 9 - 6 . 5 1 -2 . 3 4.7 33.1 - 5 1 . 8 i C 1 .6 7 .6 ! C 2C.3 - 2 1 . 6 5 C 7.1 - 7 1 6 9 0 11 .1 1 1 . 0 5 C -2 . 4 7.7 1 0 12.5 - 1 1 . I L 18 .C - 2 0 . 3 1 3 5 . 7 15.7 1 5 1 . 1 59 .1 1 4 8 . 4 4 A . 4 I -1 .1 -7.1 1 1 4 . 8 -32.2 7 C 4C .9 - 4 2 . C 7 0 7 1 . C 2 1 . 5 7 0 66.1 6 7 . 0 . 7 C 3 8 . 2 -17.2 r C 3 7 . 4 - 5 6 . 4 7 0 31.C 12.4 I 7 0 . t - 6 8 . 9 6 8 . C - 6 8 . 6 I 1 4 . C 1 1 . 4 1 3 6 . 4 3 8 .2 1 6 8 . 1 6 5 . 4 1 2 1 . 3 2 8 . 3 7 C 4 5 . i 4 4 . 0 7 C 4C .1 -4C.2 I 0 1C .1 -11.2 7 0 3 1 . 7 29.ft 7 C 2 C I 2 2 . 7 8 1 t . 5 - 4 . 9 1 4 1 . 6 - 4 1 . 1 t 4 6 . 8 - 4 6 . 3 - 8 . 6 1 2 3 . 3 - 2 1 . C 9 6 1 12 .1 1 0 . 4 -9 6 1 3 3 . 2 3 2 . B 10 6 1 4 2 . 1 4 C 3 • - 1 0 8.8 - 7 . 2 11 6 1 17 .1 - 1 6 > ' -11 6 1 * 2 3 . 2 - 2 9 . 2 . 12 A 1 1 2 . 7 - 1 3 . 4 -12 6 1 -i.i . 2 . 9 I t . 4 13.8 -*! i ' .._ ^ 2 8 . 5 2 8 . C" 14 t 1 12 .1 1 0 . 4 - 14 6 1 - 2 . 5 - 0 . 6 13 6 1 I C . l - 1 0 . 1 - 15 1 4 . ) - l * . 2 - 16 ft 1 - 2 . 1 5.1 4 6 . 6 - 4 8 . C 1 6 1 36 . f t - 7 6 . 1 4 4 . 4 4 3 . 7 2 8 1 4 1 . C 4 3 . 5 3 3 . e 33 .1 1 8 1 16 .3 1 3 . 8 -3 8 1 4 2 . 4 -40.1 4 e l 4 B . 2 - 4 4 . 1 -4 8 1 2 5 . 2 - 2 7 . 2 1 8 1 -1.4 l . C A 1 4 5 . 3 4 5 . 8 6 a l 4 5 . ft 5 0 . 6 -6 8 1 4 2 . 5 4 3 . 6 7 8 I 1 6 .1 - 1 6 . 3 -1 8 1 A C . 6 - A 3 . A 8 8 1 4 8 . 6 - 4 7 . 2 -a 8 1 1 8 . J - 2 C C 9 8 1 21 .1 21.1 - 9 8 1 39.8 4 0 . I 10 8 1 1 9 . 9 7 0 . 4 -10 e i 2 4 . 1 2 4 . 5 11 e t 2 7 . 4 - 2 6 . 8 8 1 27.7 - 2 6 . 5 17 8 1 U . 4 - 1 5 . 7 -12 a t i c e - 8 . 0 13 e t 2 1 . 2 2 0 . 4 - 13 8 1 13 .C 16.1 14 e i 1 5 . 9 1 4 . 6 S l - 2 . 1 - 2 . 2 IC 1 4 4 . 5 -46.1 1 IC 1 1 9 . C -14 . f t - 1 IC 1 24 .1 2 5 . 3 IC 1 93.1 5 3 . 7 -2 IC 1 31 .1 1 0 . 6 IC 1 - 2 . C 4.4 -3 IC t 36.8 - 3 5 . 1 4 IC 1 3 6 . 8 - 3 6 . 1 -4 IC 1 2 2 . 2 - 2 4 . 4 3 IC 1 - 2 . 1 - 4 . 6 -3 tc 1 4 5 . 3 4 4 . 5 IC 1 4 1 . C 4C.1 -6 IC 1 2 3 . 5 . 2 4 . 1 7 IC 1 1 1 . C - 1 0 . 1 - 7 IC 1 i c e - 3 1 . H IC . 1 3 5 . 2 - 3 3 . 8 -8 IC I 1 1 . 7 - 1 1 . 1 9 IC 1 11.3 15 .C - 9 IC 1 3 1 . E 12.1 IC IC 1 1 9 . 2 1 7 . C - 10 IC 1 19 .4 . 1 9 . 9 1 I IC 1 - l e . i - 1 5 . 2 - 11 IC 1 2 4 . 2 - 2 2 . 1 IC 1 2 C . 4 -14.1 -12 IC t • 9 . 2 - 9 . 9 11 IC 1 1 7 . 7 U.4 - 11 IC 1 U.4 1 5 . 2 12 1 3 5 . 3 -15.1 I 12 1 - 2 . 2 -4.1 -1 12 1 2 4 . 5 2 3 . 2 2 12 I I C C 40.1 12 1 3 3 . 3 1 0 . 2 3 12 1 - 2 . 2 1.1 -1 12 1 2 2 . * - 7 1 . 4 4 12 1 I t . 9 - 3 5 . 5 -4 1? 1 24..» -29.1 9 12 I - 2 . 3 C . 4 -5 12 1 10 .5 1 2 . 0 . 6 12 1 1 C . 2 2 1 . 9 -6 12 1 9 .5 i c e t 12 1 - 2 . 2 - f t . 9 - t 12 1 1 C 5 - 9 . 6 n 12 1 22 .1 -23.1 - 8 12 1 6.4 - 6 . 0 0 12 1 - 2 . 4 1.3 -9 12 1 15 .C 1 4 . 7 10 12 1 2 1 . 5 2 1 . 6 - IC 12 I - 2 . 4 -1.1 11 12 1 - 2 . 1 - 3 . 0 -11 12 1 2 2 . 7 -21.4 14 1 2 2 . 2 - 2 0 . 9 L 14 t 1 5 . 7 - 1 4 .C - 1 14 1 l . C 6 . 4 2 14> 1 • 1 8 . 2 1 8 . 6 14 1 I t . 3 I t . 9 14 1 11 .1 1C .2 -3 14 1 - 2 . 2 - 6 . 4 4 14 1 2 1 . 4 - 2 3 . 2 -4 14 1 13 .5 -14.4 5 14 1 - 2 . 4 3 .5 -1 14 1 1 .7 1.1 6 14 I l e . i 15 .1 -6 14 I 9 . 2 1C .6 1 14 1 I C . l - 5 . 7 -1 14 1 15 .C -13.4 14 1 - 2 . 2 - 6 . 1 -8 14 I - 2 . 2 - 6 . 7 16 1 6 .4 - 8 . 5 I 16 1 - 2 . 2 - 6 . 1 - 1 16 1 4 .6 ".1 2 16 1 7.5 8 .2 - 7 16 1 10 .1 1 1 . 2 I 2 1 1 . 2 11 .1 . 1 2 7 C . 7 6 4 . 9 -1 I 2 2 3 . 5 - 1 7 . 3 2 1 2 3 4 C 4 4 C 4 - 7 1 2 2 C ) 2 0 . 2 ] 1 2 9.1 A . C -1 1 2 - l . l C 6 4 1 2 - l . l - 2 . 6 -4 I 2 3 4 . 1 -11 .9 5 ] 2 2 7 . 5 - 2 6 . 6 -3 1 2 e .e I C . 7 16 .1 - 1 4 . 5 23.8 20.1 1 4 . 4 12.1 -21.8 - 1 . 7 A . l - 2 . 0 1.1 4 5 . 2 4 3 . 8 3.C 1 3 . C 4 3 . 9 2 C . 4 2 4 . 2 S4.) 2 2 . 6 1 3 . C -i.e I C . l 2 8 . 3 - 2 . 1 - 2 . 1 1 1 . 1 1 6 . 8 1 C 4 9.5 - 2 . 1 1 2 . C t l . J 1 3 . £ t2 . C 2 3 . 1 7 4 . 9 52. t 3 4 . 3 21.5 1 6 . e - 4 . 2 -1 .1 - 3 . 5 - 1 1 . 6 -u.e 5.7 11.4 9 4 . 8 - 4 3 . 3 41 .7 -1.4 -70.a 40.1 - 1 9 . 4 - 2 1 . 9 54 .1 - 2 3 . 3 12.7 - 2 . 6 - 1 2 . 1 35 .1 -1.1 - 2 C 6 -8.6 - 5 8 . C 2 4 . 9 7 3 . 6 42.e 41.5 3.1 -4.7 1 3 . 9 11.7 2 2 . 1 21.6 1 2 . 6 - 1 1 . 7 I t . 4 14.1 -4.A 1 6 . 2 - 1 5 . C 2 c e 11. 3 12. e -2.4 11.4 15.1 13.1 a. 4 -a.? 51.1 -49.4 86.1 85.7 35.7 -14.1 43.1 4C.4 34.9 14.1 2 2 . e -24.1 -1.1 9.4 32.5 - 3 1 . 2 36.3 -64.3 14.7 17.* 11.1 -12.6 2 1 .C 15.4 - 2 . 1 17.1 17.t - 2 . 1 11 .1 44.e 1 5 . c - 2 . 2 14. C 2 1 . 5 7 6 . 1 1 2 . 5 1.4 12 .4 4C I -42. 1 - 2 . 2 0 . 6 - 3 6 . 6 35.1 1 1 . 28.1 36.1 11.9 31. I 41.1 14.1 28.5 23.5 35 .1 -IC.7 41.6 -13.C -1.1 14.6 - 2 4 . 2 2 4 . C 10 .1 - 4 . 8 12.1 - 1 2 . 4 - 2 8 . 4 11.2 -20.1 38 .1 41 .1 -14.1 27 .1 -71.4 - 4 C 2 16.4 -11 .2 6- 4 2 4 . 5 9.) -6 9 2 31 .4 6 0 . 3 7 9 2 . 44 .9 - 4 4 . 5 -7 4 2 9 .C 7.1 6 4 2 l . C -1 . 4 - 8 9 2 1 3 . ft -32.4 4 4 i it.t 2 8 . 4 -9 9 2 14 .1 14 .C 10 9 2 - 2 . 2 -3.1 - 1 0 9 2 2 4 . 5 2 4 . 7 11 9 2 1 9 . 4 -19.2 -11 9 2 t i . e - 1 3 . 9 12 5 2 -1.! fl.2 -12 4 2 21.3 - 2 4 . 6 13 9 2 2 4 . 5 22.4 -13 4 2 - 2 . 3 2 .C -14 9 2 1 1 . 2 l t . 0 0 11 2 2 6 . 4 - 2 7 . 6 1 11 3 3 t . ) 34.1 -I 11 2 3 5 . 2 - 3 3 . 4 2 11 2 2 8 . 3 2 4 . t -2 11 2 3 2 . 3 3 2 . 8 3 11 2 2 t . l -76.2 -3 11 2 22.1 20.1 1 1 4 . 7 -15.7 -4 I t 2 3 5 . t - 3 2 . * 3 11 2 2 4 . 8 2*.2 - 5 11 2 -2.2 -4.1 6 11 2 14 .1 14.1 -6 11 7 33.1 3 3 . f 7 11 2 27.3 -25.5 "a* i t 2 -2.2 - 6 . 7 -8 11 2 2 1 . 3 -3C . 1 9 1 1 2 2 3 . 3 2 4 . 6 - 9 I t 2 -2.2 O.ft 10 U t -2 . 4 - 1 0 11 2 2 C . 4 2 0 . 8 11 11 2 22.2 . - 2 3 . 0 -11 11 2 -2 . 3 0 . 5 - 1 2 11 2 U . 4 - i e . 4 0 13 2 2 4 . C - 2 7 . 3 1 13 2 15. C 12 .4 -1 13 2 t e e -9.1 2 13 2 12 .e 1 2 . e -2 13 2 13.8 I t . A 3 13 2 2 4 , e - 2 4 . 4 -3 13 2 S . 3 11.3 4 11 2 4 .2 -r t .9 -4 13 2 15.ft - 1 9 . 3 5 11 2 2 8 . e 3 C C -5 13 2 -2.2 -5.1 A 13 2 -2 . 4 • 5.1 -6 13 2 17 .5 I t . 3 7 13 2 15 .7 - 2 C 7 -7 13 2 -2.4 2 .4 8 11 2 -2.1 2 .4 -8 12 2 22.2 - 2 1 . 1 9 13 2 14.1 13 .7 -4 13 - 1 . 3 a 15 2 17.1 - 1 2 . C 1 15 2 -2 . 3 1.? -I 19 2 -2 , 3 -0.2 2 15 2 -2.1 6.1 -2 15 2 14.« i i . a J 15 2 2 C . 1 - 1 9 . 6 4 15 2 -2.7 -1.1 -4 15 7.1 - A . C 5 15 2 1 8 . ft 1 9 . 1 -1 15 2 -2.1 - l . C 0' 2 3 24 .C 2 1.1 1 2 3 11. C - 8 .4 -1 2 3 53 .2 - 5 C . C 2 2 .1 12.ft -11.1 -2 2 i 2 1 . e -20.1 3 2 3 1 1 . 7 -12.•> -1 2 3 71 .1 6 7 . a 4 2 1 1 1 . 3 2 7 . 1 -4 2 3 It.1 27 . 1 3 2 J 11.| 55.2 -1 2 3 1.C -1.4 6' 2 1 12 .7 I t .C -6 2 3 4.3 9 . 1 1 1 1 3 4 . 5 - i e . e -7 2 3 -2 .C 0 .4 e 2 1 11.i 14 .1 -8 2 1 -2.1 3.1 4 2 3 l e . i 1 5 . 6 -4 2 1 l d . C - 1 7 . 4 10 2 1 2 1 . 3 - 2 C . 4 -io i 3 -2. 3 -1. 1 I t 2 3 -2.2 4. i -11 2 3 7 . t -7.1 12 2 3 1.1 -1.4 -12 i 3 - 2 . 5 -2 .4 11 2 ? 11.2 - 1 5 . a -13 2 3 -2 . 5 -4.ft 14 2 1 -2 .4 -1 .1 -14 2 3 U . t 15.4 11 2 1 -2.2 6.1 -15 2 1 -2 . 4 1.4 - t t 2 1 U . t -14.1 C 4 3 - 1 . 3 3.8 I 4 3 3 4 . 5 31.2 -I 4 3 11.t - 3 7 . 4 2 4 J 3 4 . 3 -21. 3 -2 4 1 1 1 . 4 11 .C 1 4 3 5 1 . 7 -14.1 -3 4 1 4 1 . t 4 C . 4 4 4 3 i e . 7 20.1, -4 4 1 1 2 . C I C 4 5 4 1 2 2 .5 2 5 . t -5 4 1 22.t -21.1 6 4 3 25.2 - 2 1 . 4 -6 4 i - i . e - 5 . 4 1 4 1 - 1.5 -2.1 -7 4 3 42 .2 4 C 2 1 2 3.4 2 1 . 3 -6 4 1 t e . p - 1 9 . t 4 4 • 1 I 3.8 1 2 . 6 -9 4 1 I t . ' -18.1 IC 4 3 U . 4 - 2 8 . 1 -10 4 1 -3 .1 5 . t 11 4 i - l . l -4.2 -11 4 3 1C.4 U.4 12 4 i 1 2 . e 2 0 . 3 -12 4 3 12 .3 -12.4 25 -Table VII - cont. Continued:-h k l F 0 3 -2.5 -1.5 -13 4 3 -7.5 — 4 . fl 3 lC .4 -11.5 - 1 * 4 ) 17.4 16.7 la 4 -2.1 3.C -15 4 i U . C 10.8 -16 4 11.I -11.C 6 ! -1 .7 2.4 38.4 39.T -1 a 8C.4 -77.5 2 6 43.1 -42.1 -2 c 12.C -13.C 3 a 27.1 -26.0 -3 e 57.2 59.9 28.? 77.3 -4 t i it.i -77 . 9 5 t 18.1 19.3 -5 6 31.3 -36.3 6 8 21.3 -19.6 -6 6 12.5 17.2 18.5 -Ifl.C -7 4 34. ft 34.5 fl 8 28.3 2H.2 fl.C -6.C 9 6 15.9 15.7 -9 t 21.C -22.3 29.9 -2/.8 -10 13.5 14.7 11 t -2.2 -6.2 -11 ft 3C.5 30.C 12 ft 29.2 28.9 -12 a 15.8 -16.3 -2.4 -4.5 -13 t 1/.5 -18.2 t 19.4 -18.3 -14 6 2C.9 19.5 -15 6 8.3 B.7 B 27.6 28.C I 8 65.6 64.2 -I a 66.4 -65.3 2 s 21.2 -72.5 -2 a 32.4 -31.4 8 45.7 -45.4 - 3 8 53.1 54.9 4 25.C 29.3 . -4 e 9.4 10.7 9 e 4C .2 19.7 -5 e 42.7 -47.? e 17.2 -19. 1 -6 8 9.4 11.2 7 8 2 l . t -7 . C. -7 e 22.C 70.7 a (t 17.9 17.9 -a 8 12.5 - U . C 9 e -2.2 0.1 -9 17-3 -18.5 -IC * a 21.C -70.S -10 e U . I 17.C a -2.4 -5.4 - 11 e 14.5 15.6 12 8 72.4 27.4 -12 t 19.4 -19.4 13 B -2.2 4.9 • -13 8 13.3 -12.6 8 17.7 17.2 IC 31.e 29.4 1 IC 5C.2 47. <3 - I IC 42. 7 -41. 4 2 IC I C R 1 .7 -2 IC 11.2 - U . C 3 IC J4.4 -J2.2 -3 tc J7.4 10.8 IC 1 J.C • lfc.1 -4 IC 1.3. 11.9 tc 78.1 2H.9 -5 IC 4C.4 -45.2 6 IC 24.7 -24.4 IC 13.C 11.9 7 IC 19.C -19. t -7 10 76. 6 24.6 e IC 2C.4 18.8 -8 tc I t .3 -17.t 9 IC -2.4 5.4 -9 IC 17.7 -15.9 10 tc 22.C -22.2 -10 IC 13.5 1 3.5 1 > tc -2.2 -7.4 - U tc 11.9 12.1 • -12 tc 16.2 - 5.7 c 12 1 -2.2 1.5 1 12 18.3 20.5. -1 12 24.2 -72.8 2 12 19.4 -17.1 12 -2 .2 2 C 12 14.5 -14.C -3 12 75.C 74. 1 17 19.2 U . C -4 t i 15.6 -12.7 9 12 13.C 12.3 - 3 12 29.7 -29.8 6 12 2C.1 -19.C -6 12 7.7 5.7 7 12 13. 4 -14.5 -7 12 ?e.i 1C.2 12 23.7 74. 1 -B 12 -2.4 -7.7 9 12 9 . 7 U . 3 - 9 12 19.C -17.1 - l c 12 13.4 11-4 14 -2 .4 -2.3 1 14 13.C 11.C -1 14 -2.4 -7.5 2 14 11.1 -10.1 -2 14 -2.4 4 4 14 2 C ? -20.1 -3 14 3 9.9 10.8 4 14 12.5 14.1 -4 14 -2 .3 -J.J 3 14 -2.2 9.8 -5 14 IJ.5 -11.7 Is -2.i -0 1 _ _ 7 14 t e . i 19.1 0 1 20.4 7 C 7 1 1 13.7 -13.3 -1 1 14.7 1 7.2 7 1 -1 .7 5.9 -2 1 l l . ! - l l . l 3 1 fc l l . l -17.3 -1 1 21.6 74.7 4 1 13.3 13.3 -4 | 11.8 19.9 5 1 IC.6 9.9 -3 I IC.3 6 1 ice - I C S -6 1 I t .7 -11.A 7 1 7.9 - l . l -7 1 fc -2.1 C.2 8 1 25.6 24.5 -0 1 5.3 8.3 9 1 5.C 2.2 -9 1 -2.3 -5 .7 10 1 -2.2 C.C -10 1 -2.4 C . l 11 t 27.C 7.7 - l l 1 - i i : -2.C 1? 1 IC.3 - IC.T -12 1 -2.5 -7.7 11 1 -2.4 -4.1 -13 1 8.8 - 9 .C 14 1 -2.2 -1.5 -14 I -2.4 - 0 . 1 -15 1 -2.1 2.1 0 1 47.5 46.5 1 » 15.) -19.1 -1 I 2*.4 21.8 7 I 33. J -H.fc -7 3 15.4 7C.7 } 3 -1.8 -7.9 -1 3 8.6 9.3 4 3 18.1 36.9 -4 ! I C l 17.1 5 * -1 .5 -4.fc -5 3 fc 12.5 -11.7 6 I 23.1 -7J.C - 3 22.8 -19.F) 7 1 I C E IC.ft -7 1 5.8 9.3 8 i 14.£ 7C.5 -8 I 21.2 19.5 * I -2.2 1.7 -4 3 31. C -17.3 10 3 IC.ft -1C.7 - IC 3 7.7 - 1 C B 11 1 -2.2 4.1 - l l 3 17.7 IG I 12 1 fc -2.5 - l . t -12 2 -2.5 2.C 13 1 fc 14.8 -13.7 -11 3 9.4 -1 .3 14 3 -2.2 -.1. 1 -14 ; -2.4 C . l -15 3 -2.2 5.9 0 5 19.8 15.4 I 5 It.2 -9.4 -1 5 fc -1.8 2.2 2 3 52.4 -54.5 -7 5 fc 44 J -46.6 1 5 19.5 17. C -3 5 fc l t . t 17.C • 4 3 fc 12.7 33.1 -4 5 fc 26-C 75.5 5 5 fc IE.5 -IB.3 -5 5 fc 22.2 -21.4 * 6 5 fc -2.1 10 5 -6 5 fc 17.7 -16.1 7 ) fc IC. 7 IC.9 -7 5 fc 22.4 77.1 8 * fc t6..> 17.C -fl 3 13.5 1 '.'.£. •i 5 * 5.1 -(..1 -9 9 fc 21.1 -21.9 10 5 fc 2 C 1 -11.1 -10 5 fc 11.7 -14.5 11 5 fc 11.5 11.9 -II 5 fc 25.1 75.5 12 5 11.1 14.2 -12 5 fc 12.1 14.2 13 5 fc 18.6 -Irt.Z -13 5 fc 17.6 -16 .5 -14 5 fc -2.1 -2.2 C 7 fc 35.2 51.7 t 7 fc 7.1 -6.2 -t 7 fc 12.4 -12.C 2 7 33.7 -51.1 -2 7 fc 54.1 - # I . B 1 7 fc 9.8 9.1 -1 7 fc 2*.6 2*.4 4 7 * I C ! 10.6 -4 7 4 33.6 11.4 5 7 fc 21.2 - n . e -5 7 fc 2 3.'. -2C.9 fc 3C.1 -77.5 -6 7 4 23.1 -76.0 7 7 4 IC.5 • 7.3 -7 7 4 2 C 4 19.3 B 7 4 25.4 28. 1 -8 1 4 15.* 15.9 9 7 * 11.7 -12.3 -4 7 4 -2.2 -7.1 IC 4 14.4 -15.7 -10 7 I C C -8.4 It 7 4 27.7 21.2 -II 7 4 7 C f 2C.8 12 7 4 tC.4 I C C -12 7 9.* 9. 7 -11 7 4 28.1 -27 . t 0 5 4 64.2 62.7 1 9 4 2 C 1 19.8 -1 fl 4 13.2 -14.C 2 5 4 41.8 -42.1 -2 9 4 37.5 -31.5 1 9 4 tC.4 tC.3 4 I 4 37.4 35.4 4 2j .< 27.C 5 9 4 11.2 -13.6 -3 ' 9 4, 14.1 -16.1 6 9 4 27.6 -75.4 -6 9 4 26.3 29 C 7 . 5 4 13.6 15.5 -7 9 4 12.8 U . C 8 9 « 18.C 18.4 -8 9 4 1 7.4 16.3 4 4 18.4 -1 7.4 -9 5 * 19.8 -?C. 1 10 9 < C 5 -14.2 4 4 -2".4 -r.4 . 11 9 * 13.« 1 3.C - 1 t 9 ' 4 24.1 74.1 9 4 -2.2 4.7 l l * 22.5 73.2 t 11 * -2.2 - l . l - 1 l l 4 -2.2 -4.ft 2 It 4 24.1 -74.4 -2 11 4 25.7 -27.C 3 11 4 7.5 7.8 -3 11 * I C C 8.2 4' 11 4 3 c ; 27 6 -4 11 4 32.C 29.9 3 1 1 4 -2.2 -1 2 * -5 11 4 -2.2 -16.8 6 11 < 27.6 -29.2 -6 t 1 4 19 ; tp .e • 7 11 4 13.5 13.2 -7 11 4 4.1 17.fi 8 t l 4 17." 1 7.5 -8 11 4 12.4 12.4 9 U 4 5 4 -17 . 9 -9 1 t * 17.1 -14.9 -10 I 1 4 5.; -9.1 0 13 4 1 7.5 1 12 4 -2.4 -4.6 2 13 * 17.5 -17.5 -7 13 4 19. 1 - 19.4 3 11 * -2.1 0.6 -3 12 * U . 3 12. C 4 13 * 17.1 18.4 -4 13 « 15.7 t7.C 5 13 ' -2.2 -7.3 -5 12 7.2 -4.9 -6 13 « 12 7 - 1 » . 1 -7 13 4 15.5 16.2 0 ; -1 1.8 I 7 1 7C.4 -19.5 -1 2 - 1.5 1.8 2 2 -1 .5 -1.6 -Z 2 -1.5 6. S 1 2 28.1 22.7 -3 2 -1.5 -4.5 4 2 11.2 11.5 -4 ; ice I C C * 9 2 5.4 -25.7 -5 2 -2 C - C 4 # 6 2 11.3 27.3 • -6 2 14.6 -11.3 7 2 - 7.C 9.C -7 2 4.9 9.3 8 2 8,7 -8.5 -8 i 15.2 lb 8 9 2 -2.2 -5.C -9 2 12.4 -:14.7 ' 10 2 -2.2 -C.« - IC 2 25.1 -10.4 1 1 2 t'..1 12.3 -11 2 11.2 -IC.6 12 i -2.3 -1.4 -12 2 8.7 4.5 -13 2 -2.4 6.7 -14 2 -2.2 -4.4 C 4 -2.C l.l 1 42.8 -41.7 -t 4 14.6 16.7 2 4 8.5 - I C ? -2 4 3C.7 - l l . l 3 4 55.8 57.1 -1 4 -2.C -4.1 4 4 -2.1 - t . e -4 4 23.8 73.4 5 4 31.4 -27.4 -5 4 9.9 10.3 6 4 5.8 8.1 -t 4 IC 6 - IC Hi 7 4 I 14.« 1 1.7 -7 4 14.4 - 14.2 a -2 2 6.5 -B 4 25.C 24 .1 9 4 7.5 -6.8 -9 4 -2.2 5.3 10 4 5 -2.5 -5.4 -10 4 15.4 -17.5 I I 4 5 -2.4 6.2 -It 4 i -7.2 ' C.4 12 4 1C.4 -fl.C -12 4 1 11.5 14.2 -13 * -2.1 -1.1 -14 4 I 9.4 -10.5 . 0 6 5 71.1 16.5 1 6 5 49.2 -41.1 -1 4 > 51.1 3 C 4 2 6 S 13.4 -11.1 -2 6 5 1 C 2 -29.7 3 6 5 24.2 25.1 -3 e 5 22 .2 -71.1 4 6 5 -2.2 C. 7 -4 6 5 24.2 25.C 4" 6 ! n.i -24.1 -5 6 5 13.4 14.1 -XI 6 5 -2.4 -4.4 -10 8 5 25.C -24.8 -11 e 5 -2.1 -0.5 -12 8 5 17.4 19.2 C IC 9 15.C 15.5 I IC 9 14.6 -15.9 -I IC 9 12.2 l l . l 7 IC 9 -2.2 - 5 . J -7 tc 3 19.7 -1 2 I IC 5 12.1 31.6 -3 IC S 2S.3 -72.1 4 tc 9 -2.5 2.9 -4 IC 5 18.1 16 4 5 tc 9 28. 1 -76. 1 -5 tc 5 11.1 13.4 6 IC 5 -2.4 7.8 -6 IC 5 73.C -21.6 7 IC 5 24.4 26.C -7 IC 3 11.8 -14.5 e IC 9 -2.2 -5.7 -fl IC 5 25.4 72.6 - 9 IC 5 -2.2 5.4 -10 IC 3 16.4 -17.1 C 13 3 12.1 U. f l 1 12 18.8 -19.4 -1 . 12 5 30.5 7M.3 2 13 3 15.5 -14.8 -2 12 3 8.3 -8.3 3 12 5 I C l 11 .3 -? 12 3 19.2 -17.6 4 13 3 -2 .2 3,5 -4 12 5 13.4 12.8 5 12 S. 15.C - 4.9 -5 13 5 12.5 1 1.8 -6 12 5 14.7 -15.C -5 8 3 16.8 15.7 • - 6 8 5 -2.2 2.9 -6 a 5 28.6 -26.6 7 8 5 28.1 21.5 -7 8 I C C -1C.6 a e •i a . ; -8.7 -a e 3 24.8 24.7 9 8 4 24.4 -25.2 - 9 e 5 8.7 a.5 10 E 5 -2.7 5 6 -12 6 5 71.2 If. 3 -13 4 5 -2.1 . - C 7 0 •» 5 21.1 ?t.r. i a 27.2 -76.1 -1 e 3 t2.4 17.7 2 8 5 7.C 4.4 -2 8 5 21.2 -21.4 3 a 5 U . C 13.9 -3 8 5 15.C -2C.4 4 e S -l.l -0.4 -4 e 5 2C.5 ?1.7 •t 8 5 14.9 -32.7 -7 4 5 -2 .2 - .1 8 4 5 -2.2 -4.C -a 6 3 19.4 7C 6 9 6 5 28.« -27,1 - 9 4 5 7.1 a.c 10 6 5 -2.4 5.7 - l o e5 15.8 -71.7 11 6 15.7 14.4 6 6 5 7.S -7.6 -6 6 5 18. 1 -19.7 7 6 5 75.C 24 .4 0 I *• -2.1 6 -2.1 C 5 -1 1 7 I 4 -2.1 6 I C * 5,4 -2 1 4 -2.1 1.1 1 1 6 -2.2 0.* -1 I 4 -2.4 -4 4 1 6 7.C -6.3 -4 "1 4 -2.4 •5.C 5 I fc e.7 -6.4 . -5 I 6 -7.4 1 2 6 1 6 14.1 14.2 -6 1 -2.5 -5.4 7 I 4 l .t . 5.9 -7 | 6 J .7 - I C 4 a i 4 -2.2 -5.1 -8 1 4 -2.5 . -6.4 9 I 6 -2.4 1.8 - 9 1 - 2 . * 4,4 10 1 * -2 ,1 C .9 - IC 1 6 -2.5 -4.1 11 1 4 -2.2 -4 . i -11 1 6 -2.4 -1.7 -12 1 i -2.3 1.7 -13 I ft 7.7 7.8 0 J 6 11.7 -11.8 I 1 ft 24.9 - I C 1 -I 2 6 21 .1 20.5 2 3 ft 5.1 K . I -2 J 5 -2.1 C f l 3 2 6 5.2 9.2 - 3 1 6 -2.2 -3.2 4 1 6 15.2 -18.5 -4 J 4 -7.2 5.1 5 1 6 2 2 5 -S 1 t -2.2 0.4 6 1 4 28.3 71.8 -fc 3 6 7 1 6.1 7 3 6 -2.2 C . l -7 1 4 17. 7 -17.1 fl 3 t 8.1 -7.6 -a i fc - 2 .7 -2.8 9 1 6 -2.4 7.4 - 9 2 4 16.7 16.1 10 3 6 12.5 1 5 -10 2 4 - 2 . " -7,5 1 I e IS .4 -16.-9 " -12 , 3 ft -2 .1 5.2 0 5 6 16.e -16.2 1 5 2 ,C -71.8 -1 5 6 79.4 28.7 2 5 4 4'.5 9.5 -2 5 6 -2.2 4.2 3 5 t te .7 18.1 -3 5 6 15.5 -1-4.1 4 5 4 2 3 , ; 74. -4 5 " 6 7.1 -5.1 5 5 4 1.5 -4.5 -5 ! 6 23 125.4 A 5 6 2C.7 l<5.5 -6 5 1C.C I C C 7 5 6 -2.5 - C . l -7 5 29 1 -27.5 a i 6 15.6 -14.8 6 -2.2 3.5 9 9 6 - 2 .3 -I., l - 9 9 6 1 7 . ; 18.B10 5 6 13.4 14.7 -10 9 ft -2.4 -1.7 -11 5 ft 14.5 -14 7 -12 5 i -2.1 3.B 0 7 6 4.4 -8.S 1 7 7.9 -8.3 -1 7 6 te . c 17.9 2 7 6 21.4 22.4 - 7 6 l l . l 13 6 3 7 6 U . 2 1C.4 -3 7 t 26.4 -77.7 4 7 6 26.1 -25.7 -4 7 6 1.8 - C t t 15.C -14.8 -5 7 6 31.5 I C R 6 7 6 24.1 21.5 - ft -2.3 -4,9 7 7 ft -2.1 T.C -7 7 6 74.8 -77. f n 7 6 72.1 -23 . C -fl 7 6 -2.4 -1.7 9 7 fc 15.4 70.8 - IC 7 h -2 .7 -1.5 5 * 12.1 -1 1.4 I 5 6 15 .£ -IB.7 -1 9 6 1 7.E 16.4 2 5 6 19.4 7 C 3 1C.4 8,8 1 9 6 l.t T.C -1 9 8 22.7 -23.2 4 5 6 2C.3 -7C.9 --2.4 -4.1 5 5 6 -2.3 -2.9 -5 9 ft t e . i lK.t 6 5 f 24. 1 27.2 -4 5 4 -2.4 - 1 . 1 7 9 ft 73 C -22.P -8 9 4 -2.2 C.J t 1 6 12.2 - IC I I 11 6 ll.l -ll.l - i U • C te c 16.2 1 I 6 14.1 15. C -2 1 1 6 -2 2 3 3 1 ft 13.5 U . 5 Z; ll J -2.2 -2.2 -19.9 -7.3 -5 It * 15.1 19.2 c 1 7 12.7 - n . 8 -2.2 -4.5 -1 2 1 -2.2 .C 2 2 1 13.2 I C 2 11.7 11.* 1 2 7 -7.2 *.c I C 4 4 2 * -7.2 -2.1 -4 i 7 1 j"i -12.C ' -5 2 \ ?.7 -). 1 -6 2 7 -2.4 14.1 1.9 U.C 7 2 7 > -I:.? -7 2 7 -2.5 5.2 -7.2 7.4 -f> 2 7 1C.2 - U . 5 •9 2 I -2.4 1.1 -10 i 7 7.3 ,! ,C 19.7 I 4 1 -l.t t .7 - 1 4 7 -2.2 1.5 7.C 7 C It .c 16.7 3 4 7 -2.2 -4 .4 -2.3 7.2 4 4 7 12.2 - i c . - ; -4 4 1 ll.l - 1 ?.4 I S ' IC.7 tC.'! 4 t fl. t -6 4 7 17.5 11 .C 15.7 -7 4 7 -7.4 -1.1 -8 4 7 ii.; -11.4 9 ? .f I .5 -10 4 1 £ . 1 4.4 0 U.C - C . " . j \ ! 8.4 - 7 . ; 5.P -1.4 1 >.\ I i . fi--7 6 7 14.1 ll.9 . ] I t -i .* 2.1 17.3 -17.7 -4 t 7 21.1 -7C.5 \i.f. 1 i.C 7 .r. 6 7 12 .8 12.C -6 6 7 32 .1 22.2 5.4 -IC.4 -n 4 7 14. i -14.5 -L5.4 l * ' -2.3 4.6 ~2 E 1 2 ; . i 74.7 -3 e 7 2C. 7 17,9 3 e 7 U . C -11.7 ~l I 7 7.i 14.2 -14.7 -4 8 7 22.1 -72.9 5 8 7 -2.2 2.C -6 •j 7 15. 7 19.r 2 ) 8 -2.2 -C.2 1 ! -2.4 f l 1! « l.l -2.3 - t n . i 7.1 ~\ 1 3 -2.4 -2.2 1.4 0.4 9.2 4 • ' i i -2.2 0. 1 -4 1 8 -7.1 c? -5 1 8 C I - 7.4 -6 t 3 -1.2 4.C - 7 1 .1 -2.2 2.C 3 1 -2.3 -5,4 _! j 8 11.1 - 14.2 -2 3 8 1.4 6.4 i e -2.2 -6.4 -1 3 8 13.7 11.5 4 1 •! -2.1 t, » -4 i a -2.3 -*>. H -•, 3 8 e.7 -10.9 -6 ? 5 4.5 it.i ; a -2.7 - 1 .9 1 » 8 12 .8 1 J.4 5 n 5 . 1 - C 6 S « -2.1 1 .C -2 3 8 -2.3 4.C - 3 9 8 11.5 15.7 -4 9 8 -2-2 - 1. -5 5 8 17.1 - U . 5