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Quantum Coherence in Light-harvesting Energy Transfer Cao, Jianshu
Description
Quantum coherence in light-harvesting complexes is explored in a minimal model of V-shape
three-level system. We systematically solve the model to predict both its transient and steadystate
coherences and demonstrate the interplay of exciton trapping at the reaction center and
the non-canonical distribution due to the system-bath coupling [1,2]. Further, we analyze the
efficiency and energy flux of the three-level model and show the optimal performance in the
intermediate range of temperature and coupling strength, consistent with our understanding of
quantum heat engines. [3] Finally, if time allows, we will explain how to generalize the above
analysis to complex light-harvesting networks using the waiting time distribution function [4].
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[1] Can natural sunlight induce coherent exciton dynamics Olsina, Dijkstra, Wang, Cao,
arXiv:1408.5385 (2014/2019)
$$
$$
[2] Non-canonical distribution and non-equilibrium transport beyond weak system-bath
coupling regime: A polaron transformation approach. D. Xu and J. Cao, Front. Phys. 11, 1
(2016)
$$
$$
[3] Polaron effects on the performance of light-harvesting systems: A quantum heat engine
perspective. D. Xu, C. Wang, Y. Zhao, and J. Cao, New J. Phys. 18, 023003 (2016)
$$
$$
[4] Correlations in single molecule photon statistics: Renewal indicator. J. Cao, J. Phys.
Chem. B, 110, 19040 (2006)
Item Metadata
| Title |
Quantum Coherence in Light-harvesting Energy Transfer
|
| Creator | |
| Publisher |
Banff International Research Station for Mathematical Innovation and Discovery
|
| Date Issued |
2019-08-20T13:31
|
| Description |
Quantum coherence in light-harvesting complexes is explored in a minimal model of V-shape
three-level system. We systematically solve the model to predict both its transient and steadystate
coherences and demonstrate the interplay of exciton trapping at the reaction center and
the non-canonical distribution due to the system-bath coupling [1,2]. Further, we analyze the
efficiency and energy flux of the three-level model and show the optimal performance in the
intermediate range of temperature and coupling strength, consistent with our understanding of
quantum heat engines. [3] Finally, if time allows, we will explain how to generalize the above
analysis to complex light-harvesting networks using the waiting time distribution function [4].
$$
$$
[1] Can natural sunlight induce coherent exciton dynamics Olsina, Dijkstra, Wang, Cao,
arXiv:1408.5385 (2014/2019)
$$
$$
[2] Non-canonical distribution and non-equilibrium transport beyond weak system-bath
coupling regime: A polaron transformation approach. D. Xu and J. Cao, Front. Phys. 11, 1
(2016)
$$
$$
[3] Polaron effects on the performance of light-harvesting systems: A quantum heat engine
perspective. D. Xu, C. Wang, Y. Zhao, and J. Cao, New J. Phys. 18, 023003 (2016)
$$
$$
[4] Correlations in single molecule photon statistics: Renewal indicator. J. Cao, J. Phys.
Chem. B, 110, 19040 (2006)
|
| Extent |
38.0 minutes
|
| Subject | |
| Type | |
| File Format |
video/mp4
|
| Language |
eng
|
| Notes |
Author affiliation: Massachusetts Institute of Technology
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| Series | |
| Date Available |
2020-09-05
|
| Provider |
Vancouver : University of British Columbia Library
|
| Rights |
Attribution-NonCommercial-NoDerivatives 4.0 International
|
| DOI |
10.14288/1.0394210
|
| URI | |
| Affiliation | |
| Peer Review Status |
Unreviewed
|
| Scholarly Level |
Faculty
|
| Rights URI | |
| Aggregated Source Repository |
DSpace
|
Item Media
Item Citations and Data
Rights
Attribution-NonCommercial-NoDerivatives 4.0 International